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基于水热柚子皮和还原氧化石墨烯的高性能三维气凝胶作为水/油分离的高效吸附剂

High-Performance Three-Dimensional Aerogel Based on Hydrothermal Pomelo Peel and Reduced Graphene Oxide as an Efficient Adsorbent for Water/Oil Separation.

作者信息

Li Dandan, Huang Jiwei, Huang Langhuan, Tan Shaozao, Liu Ting

机构信息

Guangdong Engineering Technology Research Centre of Graphene-Like Functional and High-Performance Products and Materials, Institute of Chemistry and Materials Science, Jinan University, Guangzhou 510632, China.

出版信息

Langmuir. 2021 Feb 2;37(4):1521-1530. doi: 10.1021/acs.langmuir.0c03062. Epub 2021 Jan 21.

Abstract

In this study, HPP-RGO aerogels, which were based on a hydrothermal pomelo peel (HPP) and reduced graphene oxide (RGO), were fabricated by using a green and eco-friendly two-step hydrothermal method. The characterization results showed that the HPP-RGO aerogel was endowed with extremely low density, high specific area, robust thermal stability, good mechanical property, stable acid-alkali resistance, superior recyclability, and excellent hydrophobicity and lipophilicity. Remarkably, the typical 40%-HPP-RGO aerogel presented a preferable adsorption capacity (45-80 g·g). Moreover, continuous water/oil separation was achieved via the water ring vacuum pump. The successful preparation of the HPP-RGO aerogel endows the pomelo peel with high value-added properties and improves the comprehensive utilization of agricultural wastes. Furthermore, it would open up bright prospects for the field of oil adsorption and water/oil separation.

摘要

在本研究中,基于水热柚子皮(HPP)和还原氧化石墨烯(RGO)的HPP-RGO气凝胶采用绿色环保的两步水热法制备。表征结果表明,HPP-RGO气凝胶具有极低的密度、高比表面积、强大的热稳定性、良好的机械性能、稳定的耐酸碱性能、优异的可回收性以及出色的疏水性和亲油性。值得注意的是,典型的40%-HPP-RGO气凝胶具有较好的吸附容量(45-80 g·g)。此外,通过水环真空泵实现了连续的水/油分离。HPP-RGO气凝胶的成功制备赋予了柚子皮高附加值特性,提高了农业废弃物的综合利用率。此外,它将为吸油和水/油分离领域开辟广阔前景。

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