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基于石墨烯的催化剂上二氧化碳的电化学还原。

Electrochemical Reduction of Carbon Dioxide on Graphene-Based Catalysts.

机构信息

Instituto de Materiales y Nanotecnología, Departamento de Química, Universidad de La Laguna, P.O. Box 456, 38200 La Laguna, Santa Cruz de Tenerife, Spain.

出版信息

Molecules. 2021 Jan 22;26(3):572. doi: 10.3390/molecules26030572.

DOI:10.3390/molecules26030572
PMID:33499217
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC7866188/
Abstract

The current environmental situation requires taking actions regarding processes for energy production, thus promoting renewable energies, which must be complemented with the development of routes to reduce pollution, such as the capture and storage of CO. Graphene materials have been chosen for their unique properties to be used either as electrocatalyst or as catalyst support (mainly for non-noble metals) that develop adequate efficiencies for this reaction. This review focuses on comparing experimental and theoretical results of the electrochemical reduction reaction of carbon dioxide (ECORR) described in the scientific literature to establish a correlation between them. This work aims to establish the state of the art on the electrochemical reduction of carbon dioxide on graphene-based catalysts.

摘要

当前的环境状况要求我们针对能源生产过程采取行动,从而促进可再生能源的发展,同时还必须开发减少污染的途径,例如 CO 的捕获和储存。石墨烯材料因其独特的性质而被选中,可将其用作电催化剂或催化剂载体(主要用于非贵金属),从而为该反应提供足够的效率。本综述重点比较了科学文献中描述的二氧化碳电化学还原反应(ECORR)的实验和理论结果,以建立它们之间的相关性。这项工作旨在确定基于石墨烯的催化剂上二氧化碳电化学还原的最新技术状态。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/209f/7866188/1f5447ffa10f/molecules-26-00572-g012.jpg
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https://cdn.ncbi.nlm.nih.gov/pmc/blobs/209f/7866188/9592eda0a668/molecules-26-00572-g008.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/209f/7866188/912faffe98dc/molecules-26-00572-g009.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/209f/7866188/83caa02d3c8e/molecules-26-00572-g010.jpg
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https://cdn.ncbi.nlm.nih.gov/pmc/blobs/209f/7866188/1f5447ffa10f/molecules-26-00572-g012.jpg

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ACS Appl Mater Interfaces. 2020 Apr 8;12(14):16178-16185. doi: 10.1021/acsami.9b18091. Epub 2020 Mar 27.
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Enhanced Electrocatalytic Reduction of CO via Chemical Coupling between Indium Oxide and Reduced Graphene Oxide.通过氧化铟与还原氧化石墨烯之间的化学偶联增强电催化还原CO
Nano Lett. 2019 Jun 12;19(6):4029-4034. doi: 10.1021/acs.nanolett.9b01393. Epub 2019 May 30.
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Impact of Interfacial Electron Transfer on Electrochemical CO Reduction on Graphitic Carbon Nitride/Doped Graphene.
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Boosting CHOH Production in Electrocatalytic CO Reduction over Partially Oxidized 5 nm Cobalt Nanoparticles Dispersed on Single-Layer Nitrogen-Doped Graphene.在单层氮掺杂石墨烯上分散的部分氧化的 5nm 钴纳米颗粒上电催化 CO 还原中提高 CHOH 产量。
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