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单层 WSe₂ 中确定性单光子发射器的偏振控制

Polarization Control of Deterministic Single-Photon Emitters in Monolayer WSe.

作者信息

So Jae-Pil, Jeong Kwang-Yong, Lee Jung Min, Kim Kyoung-Ho, Lee Soon-Jae, Huh Woong, Kim Ha-Reem, Choi Jae-Hyuck, Kim Jin Myung, Kim Yoon Seok, Lee Chul-Ho, Nam SungWoo, Park Hong-Gyu

机构信息

Department of Physics, Korea University, Seoul 02841, Republic of Korea.

Department of Physics, Chungbuk National University, Cheongju 28644, Republic of Korea.

出版信息

Nano Lett. 2021 Feb 10;21(3):1546-1554. doi: 10.1021/acs.nanolett.1c00078. Epub 2021 Jan 27.

Abstract

Single-photon emitters, the basic building blocks of quantum communication and information, have been developed using atomically thin transition metal dichalcogenides (TMDCs). Although the bandgap of TMDCs was spatially engineered in artificially created defects for single-photon emitters, it remains a challenge to precisely align the emitter's dipole moment to optical cavities for the Purcell enhancement. Here, we demonstrate position- and polarization-controlled single-photon emitters in monolayer WSe. A tensile strain of ∼0.2% was applied to monolayer WSe by placing it onto a dielectric rod structure with a nanosized gap. Excitons were localized in the nanogap sites, resulting in the generation of linearly polarized single-photon emission with a g of ∼0.1 at 4 K. Additionally, we measured the abrupt change in polarization of single photons with respect to the nanogap size. Our robust spatial and polarization control of emission provides an efficient way to demonstrate deterministic and scalable single-photon sources by integrating with nanocavities.

摘要

单光子发射器作为量子通信和信息的基本构建单元,已通过原子级薄的过渡金属二硫族化合物(TMDCs)得以开发。尽管TMDCs的带隙在人工制造的单光子发射器缺陷中进行了空间工程设计,但要将发射器的偶极矩精确对准光学腔以实现珀塞尔增强效应,仍然是一项挑战。在此,我们展示了单层WSe中位置和偏振可控的单光子发射器。通过将单层WSe放置在具有纳米级间隙的介电棒结构上,施加了约0.2%的拉伸应变。激子被局域在纳米间隙位置,导致在4K温度下产生g值约为0.1的线偏振单光子发射。此外,我们测量了单光子偏振相对于纳米间隙尺寸的突变。我们对发射的稳健空间和偏振控制为通过与纳米腔集成来展示确定性和可扩展的单光子源提供了一种有效方法。

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