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评估尼日利亚中北部部分地区采矿活动导致的砷及其相关健康风险:使用蒙特卡罗的概率方法。

Assessment of arsenic and its associated health risks due to mining activities in parts of North-central Nigeria: Probabilistic approach using Monte Carlo.

机构信息

Department of Physics, University of Ilorin, Ilorin, Nigeria.

出版信息

J Hazard Mater. 2021 Jun 15;412:125262. doi: 10.1016/j.jhazmat.2021.125262. Epub 2021 Jan 30.

DOI:10.1016/j.jhazmat.2021.125262
PMID:33548784
Abstract

This study evaluates health risks associated with Arsenic due to mining activities in parts of North-central Nigeria. 306 samples of soil, water and guinea corn were collected for analysis using Atomic Absorption Spectrometry. The analysis reveals varying concentration of Arsenic that is in most cases, above the acceptable limits of consumption, signifying evidence of pollution. The estimated pollution evaluation indices indicates evidence of pollution due to the mining activities. The estimated values of the bioaccumulation factors are very low. The Average Daily Intake reveals that ingestion pathway is the dominant pathway of exposure. While most of the Hazard Index (HI) estimated for the soil and grain samples are « 1, the HI estimated for the water is ≈1. This therefore, means that the probable non-cancerous effect of Arsenic in the drinking water is high. Based on the Delphii method of classification, the Incremental Lifetime Cancer Risk ranges between level II and level III for the soil and grain samples and between level VI and level VII for the water samples within the study sites. This high cancer risks was confirmed by the mean, 5th and 95th percentiles of the cumulative probabilities using the Monte Carlo simulation.

摘要

本研究评估了尼日利亚中北部部分地区采矿活动导致的砷相关健康风险。采集了 306 个土壤、水和玉米样品,使用原子吸收光谱法进行分析。分析结果显示,砷的浓度变化不定,多数情况下超过了可接受的消费限度,表明存在污染迹象。根据污染评估指数估算,存在由采矿活动引起的污染证据。生物累积因子的估算值非常低。平均日摄入量显示,摄入途径是暴露的主要途径。尽管估算的土壤和谷物样品的大部分危害指数 (HI) 都小于 1,但估算的水的 HI 约为 1。这意味着,饮用水中砷可能产生的非致癌效应较高。基于 Delphi 分类法,研究地点内土壤和谷物样品的增量终生癌症风险在 II 级和 III 级之间,而水样品的增量终生癌症风险在 VI 级和 VII 级之间。通过使用蒙特卡罗模拟计算累积概率的平均值、第 5 个百分位数和第 95 个百分位数,确认了这种高癌症风险。

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