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表面等离子体共振激发的银纳米线上MOF涂层的光催化性能

Photocatalytic Performance of the MOF-Coating Layer on SPR-Excited Ag Nanowires.

作者信息

Chen Xi, Zhang Yanshuang, Kong Xiangyun, Yao Kun, Liu Lingzhi, Zhang Jiali, Guo Zanru, Xu Wenyuan, Fang Zhili, Liu Yongxin

机构信息

School of Materials Science and Engineering, East China Jiaotong University, Shuanggang Road 808, Nanchang 330013, People's Republic of China.

Shenzhen Zhongxing New Material Technology Company Ltd., Binhai 2nd Road 8, Dapeng New District, Shenzhen 518000, People's Republic of China.

出版信息

ACS Omega. 2021 Jan 19;6(4):2882-2889. doi: 10.1021/acsomega.0c05229. eCollection 2021 Feb 2.

Abstract

The photoactive metal-organic frameworks (MOFs) were controllably coated on the surface plasmon resonance-excited Ag nanowires in a layer manner to adjust the photocatalytic activity. The influence of the thickness of the MOF coating layer on the photocatalytic activity was investigated. A thicker MOF coating layer not only facilitated the photogenerated electron-hole separation efficiency but also provided a larger Brunauer-Emmett-Teller surface area, thus enhancing the photocatalytic activity. This work provided a new way to adjust the photocatalytic activity of the photoactive MOF.

摘要

将光活性金属有机框架(MOF)以层状方式可控地包覆在表面等离子体共振激发的银纳米线上,以调节光催化活性。研究了MOF包覆层厚度对光催化活性的影响。较厚的MOF包覆层不仅提高了光生电子-空穴分离效率,还提供了更大的比表面积,从而增强了光催化活性。这项工作为调节光活性MOF的光催化活性提供了一种新方法。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/18a3/7860077/ab0991ec174b/ao0c05229_0002.jpg

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