Innovative Waste Consulting Services, LLC, Gainesville, Florida, United States of America.
Department of Environmental Engineering Sciences, University of Florida, Gainesville, Florida, United States of America.
PLoS One. 2021 Feb 26;16(2):e0246334. doi: 10.1371/journal.pone.0246334. eCollection 2021.
A critical examination of the US Environmental Protection Agency's (US EPA's) Greenhouse Gas Reporting Program (GHGRP) database provided an opportunity for the largest evaluation to date of landfilled waste decomposition kinetics with respect to different US climate regimes. In this paper, 5-8 years of annual methane collection data from 114 closed landfills located in 29 states were used to estimate site-specific waste decay rates (k) and methane collection potentials (Lc). These sites account for approximately 9% of all landfills required to report GHG emissions to the US EPA annually. The mean methane collection potential (Lc) for the sites located in regions with less than 635 mm (25 in) annual rainfall was significantly (p<0.002) lower than the mean methane collection potential of the sites located in regions with more than 635 mm (25 in) annual precipitation (49 and 73 m3 methane Mg-1 waste, respectively). This finding suggests that a fraction of the in-place biodegradable waste may not be decomposing, potentially due to a lack of adequate moisture content of landfills located in arid regions. The results of this evaluation offer insight that challenges assumptions of the traditional landfill methane estimation approach, especially in arid climates, that all methane corresponding to the total methane generation potential of the buried solid waste will be produced. Decay rates showed a significant correlation with annual precipitation, with an average k of 0.043 year-1 for arid regions (< 508 mm (20 in) year-1), 0.074 year-1 for regions with 508-1,016 mm (20-40 in) annual precipitation, and 0.09 year-1 in wet regions (> 1,016 mm (40 in) year-1). The data suggest that waste is decaying faster than the model default values, which in turn suggests that a larger fraction of methane is produced during a landfill's operating life (relative to post-closure).
对美国环境保护署(US EPA)温室气体报告计划(GHGRP)数据库的批判性审查为迄今为止对不同美国气候条件下填埋废物分解动力学进行的最大评估提供了机会。在本文中,使用了来自 29 个州的 114 个封闭垃圾填埋场的 5-8 年年度甲烷收集数据来估算特定于站点的废物衰减率(k)和甲烷收集潜力(Lc)。这些站点约占每年向美国 EPA 报告温室气体排放量的所有垃圾填埋场的 9%。年降雨量小于 635 毫米(25 英寸)的地区的垃圾填埋场的平均甲烷收集潜力(Lc)明显(p<0.002)低于年降雨量超过 635 毫米(25 英寸)的地区的垃圾填埋场的平均甲烷收集潜力(分别为 49 和 73 m3 甲烷 Mg-1 废物)。这一发现表明,部分原地可生物降解废物可能没有分解,这可能是由于干旱地区垃圾填埋场的水分含量不足所致。评估结果提供了一些见解,这些见解挑战了传统垃圾填埋场甲烷估算方法的假设,特别是在干旱气候下,即所有与掩埋固体废物总甲烷生成潜力相对应的甲烷都会产生。衰减率与年降水量呈显著相关性,干旱地区的平均 k 值为 0.043 年-1(<508 毫米(20 英寸)年-1),508-1016 毫米(20-40 英寸)年降水量的地区为 0.074 年-1,湿润地区(>1016 毫米(40 英寸)年-1)的 k 值为 0.09 年-1。数据表明,废物的衰减速度快于模型的默认值,这反过来表明在垃圾填埋场的运行寿命期间(相对于封场后)产生了更大比例的甲烷。