Qiu Qinxi, Huang Zhiming
State Key Laboratory of Infrared Physics, Shanghai Institute of Technical Physics, Chinese Academy of Sciences, 500 Yu Tian Road, Shanghai, 200083, P. R. China.
Key Laboratory of Space Active Opto-Electronics Technology, Shanghai Institute of Technical Physics, Chinese Academy of Sciences, 500 Yu Tian Road, Shanghai, 200083, P. R. China.
Adv Mater. 2021 Apr;33(15):e2008126. doi: 10.1002/adma.202008126. Epub 2021 Mar 9.
2D materials are considered to be the most promising materials for photodetectors due to their unique optical and electrical properties. Since the discovery of graphene, many photodetectors based on 2D materials have been reported. However, the low quantum efficiency, large noise, and slow response caused by the thinness of 2D materials limit their application in photodetectors. Here, recent progress on 2D material photodetectors is reviewed, covering the spectrum from ultraviolet to terahertz waves. First the interaction of 2D materials with light is analyzed in terms of optical physics. Then the present methods to improve the performance of 2D material photodetectors are summarized, such as defect engineering, p-n junctions and hybrid detectors, and the issue of serious overestimation of the performance in reported photodetectors based on 2D materials is discussed. Next, a comparison of 2D material photodetectors with traditional commercially available detectors shows that it is difficult to balance the current 2D material photodetectors with regard to having simultaneously both high sensitivity and fast response. Finally, a possible novel EIW mechanism is suggested to advance the performance of 2D material photodetectors in the future.
二维材料因其独特的光学和电学性质,被认为是用于光电探测器最具前景的材料。自石墨烯被发现以来,已报道了许多基于二维材料的光电探测器。然而,二维材料的薄度所导致的低量子效率、大噪声和慢响应,限制了它们在光电探测器中的应用。在此,综述了二维材料光电探测器的近期进展,涵盖从紫外线到太赫兹波的频谱范围。首先从光学物理角度分析二维材料与光的相互作用。然后总结了目前提高二维材料光电探测器性能的方法,如缺陷工程、p-n结和混合探测器,并讨论了在已报道的基于二维材料的光电探测器中性能被严重高估的问题。接下来,二维材料光电探测器与传统商用探测器的比较表明,要使当前的二维材料光电探测器同时具备高灵敏度和快速响应是难以实现平衡的。最后,提出了一种可能的新型电子-离子-声子(EIW)机制,以在未来提升二维材料光电探测器的性能。