Ksenzov Dmitriy, Maznev Alexei A, Unikandanunni Vivek, Bencivenga Filippo, Capotondi Flavio, Caretta Antonio, Foglia Laura, Malvestuto Marco, Masciovecchio Claudio, Mincigrucci Riccardo, Nelson Keith A, Pancaldi Matteo, Pedersoli Emanuele, Randolph Lisa, Rahmann Hendrik, Urazhdin Sergei, Bonetti Stefano, Gutt Christian
Department Physik, Universität Siegen, Walter-Flex-Strasse 3, 57072, Siegen, Germany.
Department of Chemistry, Massachusetts Institute of Technology, 77 Massachusetts Avenue, Cambridge, Massachusetts 02139, United States.
Nano Lett. 2021 Apr 14;21(7):2905-2911. doi: 10.1021/acs.nanolett.0c05083. Epub 2021 Mar 16.
We utilize coherent femtosecond extreme ultraviolet (EUV) pulses from a free electron laser (FEL) to generate transient periodic magnetization patterns with periods as short as 44 nm. Combining spatially periodic excitation with resonant probing at the M-edge of cobalt allows us to create and probe transient gratings of electronic and magnetic excitations in a CoGd alloy. In a demagnetized sample, we observe an electronic excitation with a rise time close to the FEL pulse duration and ∼0.5 ps decay time indicative of electron-phonon relaxation. When the sample is magnetized to saturation in an external field, we observe a magnetization grating, which appears on a subpicosecond time scale as the sample is demagnetized at the maxima of the EUV intensity and then decays on the time scale of tens of picoseconds via thermal diffusion. The described approach opens multiple avenues for studying dynamics of ultrafast magnetic phenomena on nanometer length scales.
我们利用来自自由电子激光(FEL)的相干飞秒极紫外(EUV)脉冲来生成周期短至44纳米的瞬态周期性磁化模式。将空间周期性激发与钴M边的共振探测相结合,使我们能够在CoGd合金中创建和探测电子与磁激发的瞬态光栅。在退磁样品中,我们观察到一种电子激发,其上升时间接近FEL脉冲持续时间,衰减时间约为0.5皮秒,这表明存在电子 - 声子弛豫。当样品在外部磁场中磁化至饱和时,我们观察到一个磁化光栅,它在亚皮秒时间尺度上出现,此时样品在EUV强度最大值处退磁,然后通过热扩散在数十皮秒的时间尺度上衰减。所描述的方法为研究纳米长度尺度上超快磁现象的动力学开辟了多种途径。