Foglia L, Mincigrucci R, Maznev A A, Baldi G, Capotondi F, Caporaletti F, Comin R, De Angelis D, Duncan R A, Fainozzi D, Kurdi G, Li J, Martinelli A, Masciovecchio C, Monaco G, Milloch A, Nelson K A, Occhialini C A, Pancaldi M, Pedersoli E, Pelli-Cresi J S, Simoncig A, Travasso F, Wehinger B, Zanatta M, Bencivenga F
Elettra - Sincrotrone Trieste S.C.p.A., Basovizza, 34149 Trieste, Italy.
Department of Chemistry, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139, USA.
Photoacoustics. 2023 Jan 19;29:100453. doi: 10.1016/j.pacs.2023.100453. eCollection 2023 Feb.
Collective lattice dynamics determine essential aspects of condensed matter, such as elastic and thermal properties. These exhibit strong dependence on the length-scale, reflecting the marked wavevector dependence of lattice excitations. The extreme ultraviolet transient grating (EUV TG) approach has demonstrated the potential of accessing a wavevector range corresponding to the 10s of nm length-scale, representing a spatial scale of the highest relevance for fundamental physics and forefront technology, previously inaccessible by optical TG and other inelastic scattering methods. In this manuscript we report on the capabilities of this technique in the context of probing thermoelastic properties of matter, both in the bulk and at the surface, as well as discussing future developments and practical considerations.
集体晶格动力学决定了凝聚态物质的基本特性,如弹性和热性质。这些特性对长度尺度表现出强烈的依赖性,反映了晶格激发对波矢的显著依赖性。极紫外瞬态光栅(EUV TG)方法已证明能够进入对应于几十纳米长度尺度的波矢范围,这代表了与基础物理和前沿技术最相关的空间尺度,而这是光学TG和其他非弹性散射方法以前无法达到的。在本论文中,我们报告了该技术在探测物质的热弹性性质方面的能力,包括体相和表面的性质,同时也讨论了未来的发展和实际考虑因素。