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基于连续谱中的束缚态的高度可控无蚀刻钙钛矿微激光器。

Highly Controllable Etchless Perovskite Microlasers Based on Bound States in the Continuum.

作者信息

Wang Yuhan, Fan Yubin, Zhang Xudong, Tang Haijun, Song Qinghai, Han Jiecai, Xiao Shumin

机构信息

Ministry of Industry and Information Technology Key Lab of Micro-Nano Optoelectronic Information System, Shenzhen Graduate School, Harbin Institute of Technology, Shenzhen 518055, People's Republic of China.

Collaborative Innovation Center of Extreme Optics, Shanxi University, Taiyuan 030006, Shanxi, People's Republic of China.

出版信息

ACS Nano. 2021 Apr 27;15(4):7386-7391. doi: 10.1021/acsnano.1c00673. Epub 2021 Mar 17.

DOI:10.1021/acsnano.1c00673
PMID:33729762
Abstract

Lead halide perovskites have been promising materials for lasing applications. Despite that a series of perovskite microlasers have been reported, their lasing modes are confined by either the as-grown morphology or the etched boundary. The first one is quite random and incompatible with integration, whereas the latter one strongly spoils the laser performances. Herein, we propose and experimentally demonstrate a robust and generic mechanism to realize well-controlled perovskite microlasers without the etching process. By patterning a one-dimensional polymer grating onto a perovskite film, we show that the symmetry-protected bound states in the continuum (BICs) can be formed in it. The intriguing properties of BICs including a widely spread mode profile and high factor, associated with the exceptional gain of perovskite, produce single-mode microlasers with high repeatability, controllability, directionality, and a polarization vortex. This mechanism can also be extended to two-dimensional nanostructures, enabling BIC lasers with different topological charges.

摘要

卤化铅钙钛矿一直是激光应用领域颇具前景的材料。尽管已经报道了一系列钙钛矿微激光器,但其激光模式受生长形态或蚀刻边界的限制。前者相当随机且与集成不兼容,而后者则严重损害激光性能。在此,我们提出并通过实验证明了一种稳健且通用的机制,无需蚀刻工艺即可实现可控的钙钛矿微激光器。通过在钙钛矿薄膜上图案化一维聚合物光栅,我们表明可以在其中形成连续统中的对称保护束缚态(BICs)。BICs的有趣特性包括广泛分布的模式轮廓和高Q因子,与钙钛矿的特殊增益相关,产生具有高重复性、可控性、方向性和偏振涡旋的单模微激光器。这种机制还可以扩展到二维纳米结构,实现具有不同拓扑电荷的BIC激光器。

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