Dai Chenjie, Wan Shuai, Li Zhe, Shi Yangyang, Zhang Shuang, Li Zhongyang
Electronic Information School, Wuhan University, Wuhan, 430072, China.
Department of Physics, The University of Hong Kong, Hong Kong, 999077, China.
Nat Commun. 2024 Jan 29;15(1):845. doi: 10.1038/s41467-024-45284-1.
Directional emission of photoluminescence despite its incoherence is an attractive technique for light-emitting fields and nanophotonics. Optical metasurfaces provide a promising route for wavefront engineering at the subwavelength scale, enabling the feasibility of unidirectional emission. However, current directional emission strategies are mostly based on static metasurfaces, and it remains a challenge to achieve unidirectional emissions tuning with high performance. Here, we demonstrate quantum dots-hydrogel integrated gratings for actively switchable unidirectional emission with simultaneously a narrow divergence angle less than 1.5° and a large diffraction angle greater than 45°. We further demonstrate that the grating efficiency alteration leads to a more than 7-fold tuning of emission intensity at diffraction order due to the variation of hydrogel morphology subject to change in ambient humidity. Our proposed switchable emission strategy can promote technologies of active light-emitting devices for radiation control and optical imaging.
尽管光致发光是非相干的,但其定向发射对于发光领域和纳米光子学而言是一种有吸引力的技术。光学超表面为亚波长尺度的波前工程提供了一条有前景的途径,使得单向发射成为可能。然而,当前的定向发射策略大多基于静态超表面,要实现高性能的单向发射调谐仍然是一个挑战。在此,我们展示了量子点 - 水凝胶集成光栅,用于实现可主动切换的单向发射,同时具有小于1.5°的窄发散角和大于45°的大衍射角。我们进一步证明,由于水凝胶形态随环境湿度变化而改变,光栅效率的改变导致衍射级次处发射强度有超过7倍的调谐。我们提出的可切换发射策略能够推动用于辐射控制和光学成像的有源发光器件技术的发展。