Borrego-Varillas Rocío, Lucchini Matteo
Opt Express. 2021 Mar 29;29(7):9711-9722. doi: 10.1364/OE.415463.
Recent development of spectroscopic techniques based on attosecond radiation has given the community the right tools to study the timing of the photoelectron process. In this work we investigate the effect of Fano resonances in attosecond streaking spectrograms and the application of standard phase-reconstruction algorithms. We show that while the existence of the infrared coupling (ac-Stark shift) hinders the applicability of FROG-like methods, under certain conditions it is still possible to use standard reconstruction algorithms to retrieve the photoemission delay of the bare resonance. Finally, we propose two strategies to study the strength of IR coupling using the attosecond streaking technique.
基于阿秒辐射的光谱技术的最新发展为研究光电子过程的时间提供了合适的工具。在这项工作中,我们研究了阿秒条纹光谱图中Fano共振的影响以及标准相位重建算法的应用。我们表明,虽然红外耦合(交流斯塔克位移)的存在阻碍了类FROG方法的适用性,但在某些条件下,仍然可以使用标准重建算法来检索裸共振的光发射延迟。最后,我们提出了两种利用阿秒条纹技术研究红外耦合强度的策略。