Rana Farhan, Koksal Okan, Jung Minwoo, Shvets Gennady, Vamivakas A Nick, Manolatou Christina
School of Electrical and Computer Engineering, Cornell University, Ithaca, New York 14853, USA.
School of Applied and Engineering Physics, Cornell University, Ithaca, New York 14853, USA.
Phys Rev Lett. 2021 Mar 26;126(12):127402. doi: 10.1103/PhysRevLett.126.127402.
We present a many-body theory of exciton-trion polaritons (ETPs) in doped two-dimensional semiconductor materials. ETPs are robust coherent hybrid excitations involving excitons, trions, and photons. In ETPs, the 2-body exciton states are coupled to the material ground state via exciton-photon interaction, and the 4-body trion states are coupled to the exciton states via Coulomb interaction. The trion states are not directly optically coupled to the material ground state. The energy-momentum dispersion of ETPs exhibit three bands. We calculate the energy band dispersions and the compositions of ETPs at different doping densities using Green's functions. The energy splittings between the polariton bands, as well as the spectral weights of the polariton bands, depend on the strength of the Coulomb coupling between the excitons and the trions, which in turn depends sensitively on the doping density. The doping density dependence of the ETP bands and the charged nature of the trion states could enable novel electrical and optical control of ETPs.
我们提出了一种关于掺杂二维半导体材料中激子 - 三重子极化激元(ETP)的多体理论。ETP是涉及激子、三重子和光子的稳健相干混合激发。在ETP中,双体激子态通过激子 - 光子相互作用与材料基态耦合,而四体三重子态通过库仑相互作用与激子态耦合。三重子态不直接与材料基态发生光学耦合。ETP的能量 - 动量色散呈现出三个能带。我们使用格林函数计算了不同掺杂密度下ETP的能带色散和组成。极化激元能带之间的能量分裂以及极化激元能带的光谱权重取决于激子和三重子之间库仑耦合的强度,而这又敏感地依赖于掺杂密度。ETP能带对掺杂密度的依赖性以及三重子态的带电性质能够实现对ETP的新型电学和光学控制。