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准束缚态连续谱增强了单层WSe₂的二次谐波产生。

Quasi-BICs enhanced second harmonic generation from WSe monolayer.

作者信息

Ren Peiwen, Huang Zhuo, Luo Song, Liu Jia, Dong Xiaoxiang, Zhang Hua, Li Jianfeng, Yang Zhilin

机构信息

College of Physical Science and Technology, State Key Laboratory of Physical Chemistry of Solid Surfaces, Xiamen University, Xiamen 361005, China.

College of Chemistry and Chemical Engineering, State Key Laboratory of Physical Chemistry of Solid Surfaces, Xiamen University, Xiamen 361005, China.

出版信息

Nanophotonics. 2024 Jun 3;13(18):3449-3456. doi: 10.1515/nanoph-2024-0108. eCollection 2024 Aug.

Abstract

Quasi-bound states in the continuum (quasi-BICs) offer unique advantages in enhancing nonlinear optical processes and advancing the development of active optical devices. Here, the tunable robust quasi-BICs resonances are experimentally achieved through the engineering of multiple-hole Si-metasurface. Notably, the quasi-BICs mode exhibits flat bands with minimal dispersion at a wide range of incident angles, as demonstrated by the angle-resolved spectroscopy measurements. Furthermore, we demonstrate a giant second-harmonic generation (SHG) enhancement by coupling a WSe monolayer to the quasi-BICs hosted in the metasurface. Leveraging the strong local electric field and high state density of the observed quasi-BICs, the SHG from the WSe monolayer can be enhanced by more than two orders of magnitude. Our work paves the way for effectively enhancing nonlinear optical processes in two dimensional (2D) materials within the framework of silicon photonics and is expected to be applied in nonlinear optical devices.

摘要

连续统中的准束缚态(quasi-BICs)在增强非线性光学过程和推动有源光学器件的发展方面具有独特优势。在此,通过多孔硅超表面工程实验实现了可调谐的稳健准BICs共振。值得注意的是,如角分辨光谱测量所示,准BICs模式在很宽的入射角范围内呈现出具有最小色散的平坦能带。此外,我们通过将单层WSe与超表面中的准BICs耦合,展示了巨大的二次谐波产生(SHG)增强。利用所观察到的准BICs的强局部电场和高态密度,单层WSe的SHG可以增强两个以上数量级。我们的工作为在硅光子学框架内有效增强二维(2D)材料中的非线性光学过程铺平了道路,并有望应用于非线性光学器件。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/422c/11501586/0c8145565498/j_nanoph-2024-0108_fig_001.jpg

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