Suppr超能文献

通过分子模拟和机器学习的混合研究确定 Gardner 转变的非平衡临界性。

Determining the nonequilibrium criticality of a Gardner transition via a hybrid study of molecular simulations and machine learning.

机构信息

School of Chemistry, Beihang University, Beijing 100191, China.

Center of Soft Matter Physics and Its Applications, Beihang University, Beijing 100191, China.

出版信息

Proc Natl Acad Sci U S A. 2021 Mar 16;118(11). doi: 10.1073/pnas.2017392118.

Abstract

Apparent critical phenomena, typically indicated by growing correlation lengths and dynamical slowing down, are ubiquitous in nonequilibrium systems such as supercooled liquids, amorphous solids, active matter, and spin glasses. It is often challenging to determine if such observations are related to a true second-order phase transition as in the equilibrium case or simply a crossover and even more so to measure the associated critical exponents. Here we show that the simulation results of a hard-sphere glass in three dimensions are consistent with the recent theoretical prediction of a Gardner transition, a continuous nonequilibrium phase transition. Using a hybrid molecular simulation-machine learning approach, we obtain scaling laws for both finite-size and aging effects and determine the critical exponents that traditional methods fail to estimate. Our study provides an approach that is useful to understand the nature of glass transitions and can be generalized to analyze other nonequilibrium phase transitions.

摘要

明显的临界现象,通常表现为关联长度的增长和动力学的减缓,在非平衡系统中无处不在,如过冷液体、非晶固体、活性物质和自旋玻璃。通常很难确定这些观察结果是否与平衡情况下的真正二阶相变有关,或者仅仅是交叉,更难测量相关的临界指数。在这里,我们表明,在三维硬球玻璃的模拟结果与最近关于 Gardner 转变的理论预测一致,这是一种连续的非平衡相变。我们使用混合分子模拟-机器学习方法,获得了有限大小和老化效应的标度律,并确定了传统方法无法估计的临界指数。我们的研究提供了一种理解玻璃转变性质的方法,并且可以推广到分析其他非平衡相变。

相似文献

3
Dynamic Gardner cross-over in a simple glass.简单玻璃中的动态 Gardner 交叉。
Proc Natl Acad Sci U S A. 2023 Jun 27;120(26):e2218218120. doi: 10.1073/pnas.2218218120. Epub 2023 Jun 20.
4
Aging, Jamming, and the Limits of Stability of Amorphous Solids.老化、阻塞与非晶态固体稳定性的极限
J Phys Chem B. 2018 Apr 5;122(13):3280-3295. doi: 10.1021/acs.jpcb.7b09553. Epub 2018 Jan 9.
9
Universal dynamic scaling in three-dimensional Ising spin glasses.三维伊辛自旋玻璃中的普适动力学标度
Phys Rev E Stat Nonlin Soft Matter Phys. 2015 Aug;92(2):022128. doi: 10.1103/PhysRevE.92.022128. Epub 2015 Aug 19.
10
Structural evolution in the aging process of supercooled colloidal liquids.过冷胶体液体老化过程中的结构演变。
Phys Rev E Stat Nonlin Soft Matter Phys. 2014 Jun;89(6):062315. doi: 10.1103/PhysRevE.89.062315. Epub 2014 Jun 26.

本文引用的文献

1
Experimental observation of the marginal glass phase in a colloidal glass.胶体玻璃中边缘玻璃相的实验观察
Proc Natl Acad Sci U S A. 2020 Mar 17;117(11):5714-5718. doi: 10.1073/pnas.1917283117. Epub 2020 Mar 3.
4
Gardner Transition in Physical Dimensions.物理维度中的 Gardner 转变。
Phys Rev Lett. 2018 Jun 1;120(22):225501. doi: 10.1103/PhysRevLett.120.225501.
7
Absence of Marginal Stability in a Structural Glass.结构玻璃中不存在边缘稳定性。
Phys Rev Lett. 2017 Nov 17;119(20):205501. doi: 10.1103/PhysRevLett.119.205501. Epub 2017 Nov 15.

文献AI研究员

20分钟写一篇综述,助力文献阅读效率提升50倍。

立即体验

用中文搜PubMed

大模型驱动的PubMed中文搜索引擎

马上搜索

文档翻译

学术文献翻译模型,支持多种主流文档格式。

立即体验