Cui Tong, Zhang Mingqian, Zhao Yun, Yang Yuanmu, Bai Benfeng, Sun Hong-Bo
Opt Lett. 2021 May 1;46(9):2095-2098. doi: 10.1364/OL.418664.
Nonlinear nanophotonics, as an emerging field in nanophotonics, eagerly calls for experimental techniques for probing and analyzing near-field nonlinear optical signals with subwavelength resolution. Here, we report an aperture-type scanning near-field optical microscopic method for probing near-field nonlinear optical processes. As a demonstration, near-field third-harmonic generation from an anapole dark-mode state generated by a silicon nanodisk is probed and imaged. The measured results agree well with the simulations, with a spatial resolution down to $0.14{\lambda _0}$ and a sensitivity of 0.1 nW. This method provides a powerful tool for characterizing nonlinear light-matter interactions at the nanoscale, which can help, for example, to unveil crystal properties involving subwavelength defects or dislocations.
非线性纳米光子学作为纳米光子学中的一个新兴领域,迫切需要用于探测和分析具有亚波长分辨率的近场非线性光学信号的实验技术。在此,我们报告了一种用于探测近场非线性光学过程的孔径型扫描近场光学显微镜方法。作为一个示例,对由硅纳米盘产生的无偶极暗模式状态下的近场三次谐波产生进行了探测和成像。测量结果与模拟结果吻合良好,空间分辨率低至(0.14{\lambda _0}),灵敏度为(0.1)纳瓦。该方法为表征纳米尺度下的非线性光与物质相互作用提供了一个强大的工具,例如,有助于揭示涉及亚波长缺陷或位错的晶体特性。