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土耳其马拉蒂亚省农业土壤中砷和痕量金属的污染状况、潜在来源及健康风险评估:案例研究

Pollution status, potential sources and health risk assessment of arsenic and trace metals in agricultural soils: A case study in Malatya province, Turkey.

机构信息

Malatya Turgut Özal University, Doğanşehir Vahap Küçük Vocational School, Department of Aquaculture, Malatya, Turkey.

Malatya Turgut Özal University, Faculty of Agriculture, Department of Horticulture, Malatya, Turkey.

出版信息

Environ Res. 2021 Nov;202:111806. doi: 10.1016/j.envres.2021.111806. Epub 2021 Jul 30.

Abstract

We measured the concentrations of arsenic and 11 trace metals in the soils from vegetable fields in Malatya province (Turkey) and assessed health risks for residential adults and children. Also, we assessed their potential sources, contamination status and ecological risks. Median concentrations of only As, Co, Ni and Cr exceeded the world soil average values, while those of Cd, As, Ni and Cu exceeded the upper continental crust contents. Contamination factor, enrichment factor and geoaccumulation index results indicated that the study region was contaminated with Cd, As, Ni and Cu likely due to use of irrigation water contaminated with industrial wastewaters and use of fertilizers and pesticides. Also, the study region had "high potential ecological risk" for Cd, whereas "low potential ecological risk" for the other trace metal(loid)s (TMs). Factor and hierarchical cluster analyses revealed that As and Cu were from anthropogenic sources, Cd and Ni from both natural and anthropogenic sources, while other TMs from natural sources. The hazard quotient values of all TMs and total hazard index values for both children and adults were lower than the risk level of 1, indicating that non-carcinogenic health risks are not expected for residents. Also, the cumulative carcinogenic risk results were within the acceptable risk range. Our results indicated that application of multivariate statistics, pollution, ecological and health indices together provide valuable knowledge for assessing soil pollution in a particular region.

摘要

我们测量了土耳其马拉蒂亚省蔬菜地土壤中的砷和 11 种微量元素浓度,并评估了居住在该地区的成年人和儿童的健康风险。此外,我们还评估了它们的潜在来源、污染状况和生态风险。只有砷、钴、镍和铬的中位数浓度超过了世界土壤平均值,而镉、砷、镍和铜的浓度则超过了大陆地壳的含量。污染因子、富集因子和地质累积指数的结果表明,研究区域受到镉、砷、镍和铜的污染,这可能是由于使用了受工业废水污染的灌溉水以及化肥和农药的使用。此外,研究区域的镉具有“高潜在生态风险”,而其他微量元素(TMs)则具有“低潜在生态风险”。因子和层次聚类分析表明,砷和铜来自人为源,镉和镍来自自然和人为源,而其他 TMs 则来自自然源。所有 TMs 的危害商数和儿童及成人的总危害指数均低于 1 的风险水平,这表明居民不会受到非致癌健康风险的影响。此外,累积致癌风险的结果也在可接受的风险范围内。我们的研究结果表明,应用多元统计、污染、生态和健康指数相结合,可以为评估特定地区的土壤污染提供有价值的信息。

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