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通过光与物质的强耦合增强二维材料中的电荷传输。

Enhanced Charge Transport in Two-Dimensional Materials through Light-Matter Strong Coupling.

作者信息

Bhatt Pooja, Kaur Kuljeet, George Jino

机构信息

Indian Institute of Science Education and Research (IISER), Mohali, Punjab 140306, India.

出版信息

ACS Nano. 2021 Aug 24;15(8):13616-13622. doi: 10.1021/acsnano.1c04544. Epub 2021 Aug 4.

Abstract

Strong light-matter interaction of functional materials is emerging as a promising area of research. Recent experiments suggest that material properties like charge transport can be controlled by coupling to a vacuum electromagnetic field. Here, we explored the design of a Fabry-Perot cavity in a field-effect transistor configuration and studied the charge transport in two-dimensional materials. The optical and electrical measurements of strongly coupled WS suggest an enhancement of electron transport at room temperature. Electron mobility is enhanced more than 50 times at ON resonance conditions. Similarly, / ratio of the device increased by 2 orders of magnitude without chemical modification of the active layer. Cavity tuning and coupling strength-dependent studies support the evidence of modifying the electronic properties of the coupled system. A clear correlation in the effective mass of the polaritonic state and Schottky barrier height indicates a collective nature of light-matter interaction.

摘要

功能材料的强光-物质相互作用正成为一个很有前景的研究领域。最近的实验表明,诸如电荷传输等材料特性可以通过与真空电磁场耦合来控制。在此,我们探索了场效应晶体管配置中法布里-珀罗腔的设计,并研究了二维材料中的电荷传输。强耦合WS的光学和电学测量表明,室温下电子传输得到增强。在共振条件下,电子迁移率提高了50倍以上。同样,在不对外加层进行化学修饰的情况下,器件的/比率增加了2个数量级。腔调谐和耦合强度相关研究支持了改变耦合系统电子特性的证据。极化激元态的有效质量与肖特基势垒高度之间的明显相关性表明了光-物质相互作用的集体性质。

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