The Influence of Local Strain Distribution on the Effective Electrical Resistance of Carbon Black Filled Natural Rubber.

A monotonous relation between strain and measured electric resistance is highly appreciated in stretchable elastomer sensors. In real-life application the voids or technological holes of strained samples often induce non-homogeneous local strain. The present article focused on studying the effect of non-homogeneous local strain on measured direct current (DC) effective electric resistance (EER) on samples of natural rubber (NR), reinforced with 50, 60 and 70 phr of carbon black (CB). Samples were imparted geometrical inhomogeneities to obtain varied local strains. The resulting strain distribution was analyzed using Digital Image Correlation (DIC). EER exhibited a well-detectable influence of locations of inhomogeneities. Expectedly, the EER globally decreased with an increase in CB loading, but showed a steady increase as a function of strain for 50 and 60 phr over the complete testing protocol. Interestingly, for 70 phr of CB, under the same testing conditions, an alternating trend in EER was encountered. This newly observed behavior was explained through a novel hypothesis-"current propagation mode switching phenomenon". Finally, experimentally measured EERs were compared with the calculated ones, obtained by summing the global current flow through a diversity of strain dependent resistive domains.