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受限电液动力学驱动液体中非平衡模式的多样性及活性的出现。

Diversity of non-equilibrium patterns and emergence of activity in confined electrohydrodynamically driven liquids.

作者信息

Raju Geet, Kyriakopoulos Nikos, Timonen Jaakko V I

机构信息

Department of Applied Physics, Aalto University School of Science, P.O. Box 15100, Espoo FI-02150, Finland.

出版信息

Sci Adv. 2021 Sep 17;7(38):eabh1642. doi: 10.1126/sciadv.abh1642. Epub 2021 Sep 15.

Abstract

Spontaneous emergence of organized states in materials driven by non-equilibrium conditions is of notable fundamental and technological interest. In many cases, the states are complex, and their emergence is challenging to predict. Here, we show that an unexpectedly diverse collection of dissipative organized states emerges in a simple system of two liquids under planar confinement when driven by electrohydrodynamic shearing. At low shearing, a symmetry breaking at the liquid-liquid interface leads to a one-dimensional corrugation pattern. At slightly stronger shearing, topological changes give raise to the emergence of Quincke rolling filaments, filament networks, and two-dimensional bicontinuous fluidic lattices. At strong shearing, the system transitions into dissipating polygonal, toroidal, and active droplets that form dilute gas-like states at low densities and complex active emulsions at higher densities. The diversity of the observed dissipative organized states is exceptional, pointing toward non-equilibrium optical devices and new avenues in several fields of research.

摘要

由非平衡条件驱动的材料中有序状态的自发出现具有显著的基础和技术意义。在许多情况下,这些状态很复杂,其出现难以预测。在这里,我们表明,在平面限制下的两种液体的简单系统中,当由电流体动力学剪切驱动时,会出现意想不到的多种耗散有序状态。在低剪切力下,液 - 液界面处的对称性破缺会导致一维波纹图案。在稍强的剪切力下,拓扑变化会导致出现昆克滚动细丝、细丝网络和二维双连续流体晶格。在强剪切力下,系统会转变为耗散的多边形、环形和活性液滴,这些液滴在低密度下形成类似稀薄气体的状态,在高密度下形成复杂的活性乳液。观察到的耗散有序状态的多样性非常突出,为非平衡光学器件以及多个研究领域开辟了新途径。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b1e9/8443174/0d03104b7d1e/sciadv.abh1642-f1.jpg

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