Lu Yi, Zhang Hao, Fan Deqi, Chen Zupeng, Yang Xiaofei
College of Science, Nanjing Forestry University, Nanjing 210037, China.
College of Chemical Engineering, Nanjing Forestry University, Nanjing 210037, China.
J Hazard Mater. 2022 Feb 5;423(Pt B):127128. doi: 10.1016/j.jhazmat.2021.127128. Epub 2021 Sep 5.
Effectively harnessing renewable and inexhaustible solar radiation for energy conversion has attracted significant research interest in the past decade. Solar thermal conversion, as a ubiquitous phenomenon, can be implemented to evaporate water and concurrently boost photocatalytic performance for addressing freshwater scarcity and energy crisis. Most recently, solar water evaporation accompanied by photocatalytic degradation, sterilization, and hydrogen production has been proposed as a promising avenue to endow new vitality into the field of clean water and energy production. Driven by the advances of rationally designed solar-powered functional materials, a large variety of photothermal-coupled photocatalysis technologies have been exploited. In this context, it is imperative to summarize the recent progress and discuss the challenges in this multidisciplinary field. Herein, we overview photothermal materials based on various fundamental principles and highlight emerging applications in the areas of solar water evaporation, water purification, and solar-driven energy production. Furthermore, the challenges and perspectives toward both fundamental research and practical applications are also proposed. It is envisioned that this review can provide insightful suggestions to further advance the development of integrated solar thermal driven water evaporation and photocatalytic systems to fulfill concurrent energy conversion and environmental applications.
在过去十年中,有效利用可再生且取之不尽的太阳辐射进行能量转换已引起了广泛的研究兴趣。作为一种普遍存在的现象,太阳能热转换可用于蒸发水,并同时提高光催化性能,以解决淡水短缺和能源危机问题。最近,伴有光催化降解、杀菌和制氢的太阳能水蒸发被认为是为清洁水和能源生产领域注入新活力的一条很有前景的途径。在合理设计的太阳能功能材料发展的推动下,人们开发了各种各样的光热耦合光催化技术。在此背景下,总结该多学科领域的最新进展并讨论其面临的挑战势在必行。在此,我们基于各种基本原理对光热材料进行了概述,并重点介绍了在太阳能水蒸发、水净化和太阳能驱动能源生产领域的新兴应用。此外,还针对基础研究和实际应用提出了挑战和展望。预计这篇综述可为进一步推进集成太阳能热驱动水蒸发和光催化系统的发展提供有见地的建议,以实现同时进行的能量转换和环境应用。