Staps T J A, Platier B, Mihailova D, Meijaard P, Beckers J
Department of Applied Physics, Eindhoven University of Technology, P.O. Box 513, 5600MB Eindhoven, The Netherlands.
Plasma Matters B.V., Eindhoven University of Technology, P.O. Box 513, 5600MB Eindhoven, The Netherlands.
Rev Sci Instrum. 2021 Sep 1;92(9):093504. doi: 10.1063/5.0054851.
Low-temperature plasmas are widely studied in laboratory environments and form the backbone of many industrial processes. Highly energized electrons enable processes such as ionization, dissociation, and plasma chemical reactions, while the heavy species, such as neutral gas atoms and molecules, remain near room temperature. Hence, understanding the electron dynamics is crucial to the control and optimization of plasmas and their applications. In this contribution, we investigated the impact of electron density profile correction on microwave cavity resonance spectroscopy (MCRS) as a diagnostic tool for low-pressure discharges. Following standard practice, we first obtained a volume-averaged electron density by assuming a uniform plasma in the interpretation of the MCRS diagnostic technique. Second, we compare the experiments with a numerical model solved using PLASIMO software to evaluate the predictive capabilities. Third, we obtained profile-corrected electron densities by means of incorporating the numerically obtained distribution of the electron density and the numerical solution for the resonant microwave electric field in the interpretation of the experimental data using MCRS. Although the volume-averaged data agree closely with the electron density found from the numerical model, it is shown that implementing the spatial distribution of the electron density and the microwave electric field leads to a significant correction to the experimental data. The developed strategy could easily be implemented in other situations deploying MCRS as a non-invasive technique for measuring the electron density.
低温等离子体在实验室环境中得到了广泛研究,并构成了许多工业过程的核心。高能电子能够引发诸如电离、解离和等离子体化学反应等过程,而诸如中性气体原子和分子等重粒子则保持在接近室温的状态。因此,理解电子动力学对于等离子体的控制、优化及其应用至关重要。在本论文中,我们研究了电子密度分布校正对微波腔共振光谱(MCRS)的影响,MCRS作为一种用于低压放电的诊断工具。按照标准做法,我们在解释MCRS诊断技术时,首先通过假设等离子体均匀分布来获得体积平均电子密度。其次,我们将实验结果与使用PLASIMO软件求解的数值模型进行比较,以评估其预测能力。第三,我们在使用MCRS解释实验数据时,通过纳入数值获得的电子密度分布和共振微波电场的数值解,得到了分布校正后的电子密度。尽管体积平均数据与从数值模型中得到的电子密度非常吻合,但结果表明纳入电子密度和微波电场的空间分布会对实验数据产生显著校正。所开发的策略可以很容易地应用于其他将MCRS作为测量电子密度的非侵入性技术的情况。