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金沙江下游多介质中微量元素的风险评估与来源解析。

Risk assessment and source apportionment of trace elements in multiple compartments in the lower reach of the Jinsha River, China.

机构信息

State Key Laboratory of Hydraulics and Mountain River Engineering, College of Water Resource and Hydropower, Sichuan University, No. 24 South Section 1, Yihuan Road, Chengdu, 610065, China.

Changjiang Water Resources Protection Institute, Wuhan, 430051, China.

出版信息

Sci Rep. 2021 Oct 8;11(1):20041. doi: 10.1038/s41598-021-99626-w.

Abstract

Studies on trace element (TE) pollution in abiotic matrices have typically focused on water, sediment, and soil, either separately or in pairs. The importance of multi-media connectivity has been ignored. This study analyzed the concentrations of 6 TEs in three connected environmental compartments of a 28-km section of the lower reach of the Jinsha River. The ecological risk posed by TEs was higher in soil than in sediment. The contribution of exposure pathways to human health risk were ranked as ingestion > dermal contact > inhalation. An improved regional environmental risk index (RERI) method was then developed to evaluate the comprehensive risk on both ecology and human health caused by TEs. The average RERI value was generally higher in the wet season (0.42) than in the dry (0.41) and dry-to-wet transition seasons (0.08) because of the combined effects of the high TE concentrations in riparian soil and the long exposure time. Source apportionment indicated that industrial activities, weathering of parent rock, and agricultural activities were possible sources of TEs in this region. The methods and results of this study could inform local environmental management and provide references for similar cases wherein multiple compartments of river systems should be considered.

摘要

研究痕量元素 (TE) 在非生物基质中的污染,通常侧重于水、沉积物和土壤,要么单独研究,要么两两成对研究。多介质连通性的重要性被忽视了。本研究分析了金沙江下游 28 公里河段三个相连环境介质中 6 种 TE 的浓度。土壤中的 TE 生态风险高于沉积物。暴露途径对人体健康风险的贡献大小排序为:摄食>皮肤接触>吸入。然后,开发了一种改进的区域环境风险指数 (RERI) 方法,以评估 TE 对生态和人体健康的综合风险。由于河岸土壤中 TE 浓度高和暴露时间长的综合影响,雨季的平均 RERI 值(0.42)普遍高于旱季(0.41)和旱季到雨季的过渡期(0.08)。来源分配表明,工业活动、母岩风化和农业活动可能是该地区 TE 的来源。本研究的方法和结果可以为当地环境管理提供信息,并为类似情况下需要考虑河流系统多个介质的情况提供参考。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9e8a/8501140/39e10ee6d9e1/41598_2021_99626_Fig1_HTML.jpg

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