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居住区内细颗粒物中 Pb 的空间分布、污染水平及健康风险:以中国西北西安市为例。

Spatial distribution, pollution level, and health risk of Pb in the finer dust of residential areas: a case study of Xi'an, northwest China.

机构信息

School of Geography and Tourism, Shaanxi Normal University, Xi'an, 710119, People's Republic of China.

Institute of Geographic Sciences and Natural Resources Research, CAS, Beijing, 100101, People's Republic of China.

出版信息

Environ Geochem Health. 2022 Oct;44(10):3541-3554. doi: 10.1007/s10653-021-01116-5. Epub 2021 Oct 9.

Abstract

The spatial distribution, pollution level, and exposure risk of Pb in the finer dust (particle size < 63 μm) of residential areas in Xi'an, northwest China were investigated in this study. Geographical information systems and geodetector methods were used to analyze the spatial variability of Pb content in the finer dust of Xi'an and its forming mechanism. The enrichment factor was used to assess the extent of Pb pollution, and the hazard index was used to evaluate the health risks to children and adults exposed to Pb. The results showed that the average content of Pb in the finer dust of residential areas in Xi'an was 99.9 mg kg. In the Xi'an urban area, a higher Pb content was mainly found in the finer dust near the Second Ring Road of Xi'an City, and the Pb content in the old town of Xi'an City was relatively lower than that near the Second Ring Road. The results of geodetector analysis indicate that the spatial variability of Pb in the finer dust of the Xi'an urban area was primarily controlled by the interaction among vehicle emissions, daily behavior of residents, and industrial emissions. Pb in the finer dust from residential areas in all districts showed moderate enrichment. The non-cancer risks of Pb in the finer dust were within the safe range for both children and adults. However, the prolonged exposure risk of Pb in the finer dust of residential areas should be considered for children.

摘要

本研究调查了中国西北部西安市居民区细尘(粒径<63μm)中 Pb 的空间分布、污染水平和暴露风险。本研究采用地理信息系统和地理探测器方法分析了西安市细尘中 Pb 含量的空间变异性及其形成机制。采用富集因子评估 Pb 污染程度,采用危害指数评估儿童和成人接触 Pb 的健康风险。结果表明,西安市居民区细尘中 Pb 的平均含量为 99.9mg/kg。在西安市城区,较高的 Pb 含量主要出现在西安市二环路附近的细尘中,而西安市老城区的 Pb 含量相对低于二环路附近。地理探测器分析结果表明,西安市城区细尘中 Pb 的空间变异性主要受车辆排放、居民日常行为和工业排放之间的相互作用控制。各城区居民区细尘中 Pb 呈中等富集。细尘中 Pb 对儿童和成人的非致癌风险均处于安全范围。然而,应考虑儿童长期暴露于居民区细尘中 Pb 的风险。

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