McGhee Kirsty E, Putintsev Anton, Jayaprakash Rahul, Georgiou Kyriacos, O'Kane Mary E, Kilbride Rachel C, Cassella Elena J, Cavazzini Marco, Sannikov Denis A, Lagoudakis Pavlos G, Lidzey David G
Department of Physics and Astronomy, University of Sheffield, Hicks Building, Hounsfield Road, Sheffield, S3 7RH, UK.
Centre of Photonics and Quantum Materials, Skolkovo Institute of Science and Technology, Moscow, Russian Federation, 121205.
Sci Rep. 2021 Oct 22;11(1):20879. doi: 10.1038/s41598-021-00203-y.
We have developed a simplified approach to fabricate high-reflectivity mirrors suitable for applications in a strongly-coupled organic-semiconductor microcavity. Such mirrors are based on a small number of quarter-wave dielectric pairs deposited on top of a thick silver film that combine high reflectivity and broad reflectivity bandwidth. Using this approach, we construct a microcavity containing the molecular dye BODIPY-Br in which the bottom cavity mirror is composed of a silver layer coated by a SiO and a NbO film, and show that this cavity undergoes polariton condensation at a similar threshold to that of a control cavity whose bottom mirror consists of ten quarter-wave dielectric pairs. We observe, however, that the roughness of the hybrid mirror-caused by limited adhesion between the silver and the dielectric pair-apparently prevents complete collapse of the population to the ground polariton state above the condensation threshold.
我们已经开发出一种简化方法来制造适用于强耦合有机半导体微腔应用的高反射率镜子。这种镜子基于沉积在厚银膜顶部的少量四分之一波长介质对,兼具高反射率和宽反射率带宽。利用这种方法,我们构建了一个包含分子染料BODIPY-Br的微腔,其中底部腔镜由涂有SiO和NbO膜的银层组成,并表明该腔在与底部镜由十个四分之一波长介质对组成的对照腔相似的阈值下发生极化激元凝聚。然而,我们观察到,由于银与介质对之间附着力有限导致的混合镜粗糙度,显然会阻止在凝聚阈值以上粒子数完全坍缩到基态极化激元状态。