Kasprzak J, Richard M, Kundermann S, Baas A, Jeambrun P, Keeling J M J, Marchetti F M, Szymańska M H, André R, Staehli J L, Savona V, Littlewood P B, Deveaud B, Dang Le Si
CEA-CNRS-UJF joint group Nanophysique et Semiconducteurs, Laboratoire de Spectrométrie Physique, UMR5588, Université J. Fourier-Grenoble, F-38402 Saint Martin d'Hères cedex, France.
Nature. 2006 Sep 28;443(7110):409-14. doi: 10.1038/nature05131.
Phase transitions to quantum condensed phases--such as Bose-Einstein condensation (BEC), superfluidity, and superconductivity--have long fascinated scientists, as they bring pure quantum effects to a macroscopic scale. BEC has, for example, famously been demonstrated in dilute atom gas of rubidium atoms at temperatures below 200 nanokelvin. Much effort has been devoted to finding a solid-state system in which BEC can take place. Promising candidate systems are semiconductor microcavities, in which photons are confined and strongly coupled to electronic excitations, leading to the creation of exciton polaritons. These bosonic quasi-particles are 10(9) times lighter than rubidium atoms, thus theoretically permitting BEC to occur at standard cryogenic temperatures. Here we detail a comprehensive set of experiments giving compelling evidence for BEC of polaritons. Above a critical density, we observe massive occupation of the ground state developing from a polariton gas at thermal equilibrium at 19 K, an increase of temporal coherence, and the build-up of long-range spatial coherence and linear polarization, all of which indicate the spontaneous onset of a macroscopic quantum phase.
向量子凝聚相的相变——如玻色-爱因斯坦凝聚(BEC)、超流性和超导性——长期以来一直吸引着科学家,因为它们将纯粹的量子效应带到了宏观尺度。例如,在温度低于200纳开尔文的铷原子稀薄气体中,BEC已得到了著名的证实。人们付出了很多努力来寻找一个能发生BEC的固态系统。有前景的候选系统是半导体微腔,其中光子被限制并与电子激发强烈耦合,从而导致激子极化激元的产生。这些玻色子准粒子比铷原子轻10^9倍,因此理论上允许在标准低温温度下发生BEC。在这里,我们详细介绍了一组全面的实验,为极化激元的BEC提供了令人信服的证据。在临界密度以上,我们观察到在19 K的热平衡下,从极化激元气体中发展出大量基态占据、时间相干性增加以及长程空间相干性和线性极化的形成,所有这些都表明宏观量子相的自发出现。