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应变工程二维材料中的准一维激子通道。

Quasi-1D exciton channels in strain-engineered 2D materials.

作者信息

Dirnberger Florian, Ziegler Jonas D, Faria Junior Paulo E, Bushati Rezlind, Taniguchi Takashi, Watanabe Kenji, Fabian Jaroslav, Bougeard Dominique, Chernikov Alexey, Menon Vinod M

机构信息

Department of Physics, City College of New York, New York, NY 10031, USA.

Department of Physics, University of Regensburg, 93040 Regensburg, Germany.

出版信息

Sci Adv. 2021 Oct 29;7(44):eabj3066. doi: 10.1126/sciadv.abj3066.

DOI:10.1126/sciadv.abj3066
PMID:34714670
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC8555901/
Abstract

Strain engineering is a powerful tool in designing artificial platforms for high-temperature excitonic quantum devices. Combining strong light-matter interaction with robust and mobile exciton quasiparticles, two-dimensional transition metal dichalcogenides (2D TMDCs) hold great promise in this endeavor. However, realizing complex excitonic architectures based on strain-induced electronic potentials alone has proven to be exceptionally difficult so far. Here, we demonstrate deterministic strain engineering of both single-particle electronic bandstructure and excitonic many-particle interactions. We create quasi-1D transport channels to confine excitons and simultaneously enhance their mobility through locally suppressed exciton-phonon scattering. Using ultrafast, all-optical injection and time-resolved readout, we realize highly directional exciton flow with up to 100% anisotropy both at cryogenic and room temperatures. The demonstrated fundamental modification of the exciton transport properties in a deterministically strained 2D material with effectively tunable dimensionality has broad implications for both basic solid-state science and emerging technologies.

摘要

应变工程是设计用于高温激子量子器件的人工平台的强大工具。二维过渡金属二卤化物(2D TMDCs)将强光-物质相互作用与稳健且可移动的激子准粒子相结合,在这一领域极具潜力。然而,迄今为止,仅基于应变诱导的电势来实现复杂的激子结构已被证明异常困难。在此,我们展示了单粒子电子能带结构和激子多粒子相互作用的确定性应变工程。我们创建准一维传输通道来限制激子,并通过局部抑制激子-声子散射同时提高其迁移率。利用超快全光注入和时间分辨读出,我们在低温和室温下均实现了高达100%各向异性的高度定向激子流。在具有有效可调维度的确定性应变二维材料中激子输运性质的这一基本改变,对基础固态科学和新兴技术都具有广泛影响。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/00d6/8555901/42998220b7a4/sciadv.abj3066-f4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/00d6/8555901/98a4bed34257/sciadv.abj3066-f1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/00d6/8555901/5f36e6c8b551/sciadv.abj3066-f2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/00d6/8555901/e816795413d1/sciadv.abj3066-f3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/00d6/8555901/42998220b7a4/sciadv.abj3066-f4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/00d6/8555901/98a4bed34257/sciadv.abj3066-f1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/00d6/8555901/5f36e6c8b551/sciadv.abj3066-f2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/00d6/8555901/e816795413d1/sciadv.abj3066-f3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/00d6/8555901/42998220b7a4/sciadv.abj3066-f4.jpg

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2
Nonclassical Exciton Diffusion in Monolayer WSe_{2}.单层WSe₂中的非经典激子扩散
Phys Rev Lett. 2021 Aug 13;127(7):076801. doi: 10.1103/PhysRevLett.127.076801.
3
Autoionization and Dressing of Excited Excitons by Free Carriers in Monolayer WSe_{2}.单层WSe₂中自由载流子对激发激子的自电离和修饰
层状反铁磁体中的磁约束表面激子和体激子
Nat Mater. 2025 Mar;24(3):391-398. doi: 10.1038/s41563-025-02129-6. Epub 2025 Feb 19.
4
Ultrafast optical properties and applications of anisotropic 2D materials.各向异性二维材料的超快光学特性及应用
Nanophotonics. 2024 Jan 17;13(2):107-154. doi: 10.1515/nanoph-2023-0639. eCollection 2024 Jan.
5
Programmable nanowrinkle-induced room-temperature exciton localization in monolayer WSe.可编程纳米皱纹诱导的单层二硒化钨室温激子局域化
Nat Commun. 2024 Feb 20;15(1):1543. doi: 10.1038/s41467-024-45936-2.
6
Direct Imaging of Carrier Funneling in a Dielectric Engineered 2D Semiconductor.介电工程二维半导体中载流子漏斗效应的直接成像
ACS Nano. 2024 Jan 9;18(1):264-271. doi: 10.1021/acsnano.3c05957. Epub 2023 Dec 18.
7
Recent progress of exciton transport in two-dimensional semiconductors.二维半导体中激子输运的最新进展。
Nano Converg. 2023 Dec 15;10(1):57. doi: 10.1186/s40580-023-00404-3.
8
Kapitza-resistance-like exciton dynamics in atomically flat MoSe-WSe lateral heterojunction.原子级平整的MoSe-WSe横向异质结中类卡皮察电阻的激子动力学
Nat Commun. 2023 Sep 21;14(1):5881. doi: 10.1038/s41467-023-41538-6.
9
Energy transfer and charge transfer between semiconducting nanocrystals and transition metal dichalcogenide monolayers.半导体纳米晶体和过渡金属二卤化物单层之间的能量转移和电荷转移。
Chem Commun (Camb). 2023 Jun 20;59(50):7717-7730. doi: 10.1039/d3cc01125a.
10
Interface engineering of charge-transfer excitons in 2D lateral heterostructures.二维横向异质结构中电荷转移激子的界面工程。
Nat Commun. 2023 Apr 28;14(1):2438. doi: 10.1038/s41467-023-37889-9.
Phys Rev Lett. 2020 Dec 31;125(26):267401. doi: 10.1103/PhysRevLett.125.267401.
4
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Nanoscale. 2020 Oct 22;12(40):20786-20796. doi: 10.1039/d0nr04557h.
5
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Nano Lett. 2020 Sep 9;20(9):6791-6797. doi: 10.1021/acs.nanolett.0c02757. Epub 2020 Aug 24.
6
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Nat Mater. 2020 Oct;19(10):1068-1073. doi: 10.1038/s41563-020-0730-8. Epub 2020 Jul 13.
7
Heterobilayers of 2D materials as a platform for excitonic superfluidity.二维材料异质双层作为激子超流的平台
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