Dirnberger Florian, Ziegler Jonas D, Faria Junior Paulo E, Bushati Rezlind, Taniguchi Takashi, Watanabe Kenji, Fabian Jaroslav, Bougeard Dominique, Chernikov Alexey, Menon Vinod M
Department of Physics, City College of New York, New York, NY 10031, USA.
Department of Physics, University of Regensburg, 93040 Regensburg, Germany.
Sci Adv. 2021 Oct 29;7(44):eabj3066. doi: 10.1126/sciadv.abj3066.
Strain engineering is a powerful tool in designing artificial platforms for high-temperature excitonic quantum devices. Combining strong light-matter interaction with robust and mobile exciton quasiparticles, two-dimensional transition metal dichalcogenides (2D TMDCs) hold great promise in this endeavor. However, realizing complex excitonic architectures based on strain-induced electronic potentials alone has proven to be exceptionally difficult so far. Here, we demonstrate deterministic strain engineering of both single-particle electronic bandstructure and excitonic many-particle interactions. We create quasi-1D transport channels to confine excitons and simultaneously enhance their mobility through locally suppressed exciton-phonon scattering. Using ultrafast, all-optical injection and time-resolved readout, we realize highly directional exciton flow with up to 100% anisotropy both at cryogenic and room temperatures. The demonstrated fundamental modification of the exciton transport properties in a deterministically strained 2D material with effectively tunable dimensionality has broad implications for both basic solid-state science and emerging technologies.
应变工程是设计用于高温激子量子器件的人工平台的强大工具。二维过渡金属二卤化物(2D TMDCs)将强光-物质相互作用与稳健且可移动的激子准粒子相结合,在这一领域极具潜力。然而,迄今为止,仅基于应变诱导的电势来实现复杂的激子结构已被证明异常困难。在此,我们展示了单粒子电子能带结构和激子多粒子相互作用的确定性应变工程。我们创建准一维传输通道来限制激子,并通过局部抑制激子-声子散射同时提高其迁移率。利用超快全光注入和时间分辨读出,我们在低温和室温下均实现了高达100%各向异性的高度定向激子流。在具有有效可调维度的确定性应变二维材料中激子输运性质的这一基本改变,对基础固态科学和新兴技术都具有广泛影响。