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实验实现的非高斯相关棘轮中的输运与扩散增强

Transport and Diffusion Enhancement in Experimentally Realized Non-Gaussian Correlated Ratchets.

作者信息

Paneru Govind, Park Jin Tae, Pak Hyuk Kyu

机构信息

Center for Soft and Living Matter, Institute for Basic Science (IBS), Ulsan 44919, Republic of Korea.

Department of Physics, Ulsan National Institute of Science and Technology, Ulsan 44919, Republic of Korea.

出版信息

J Phys Chem Lett. 2021 Nov 18;12(45):11078-11084. doi: 10.1021/acs.jpclett.1c03037. Epub 2021 Nov 8.

DOI:10.1021/acs.jpclett.1c03037
PMID:34748337
Abstract

Living cells are known to generate non-Gaussian active fluctuations significantly larger than thermal fluctuations owing to various active processes. Understanding the effect of these active fluctuations on various physicochemical processes, such as the transport of molecular motors, is a fundamental problem in nonequilibrium physics. Therefore, we experimentally and numerically studied an active Brownian ratchet comprising a colloidal particle in an optically generated asymmetric periodic potential driven by non-Gaussian noise having finite-amplitude active bursts, each arriving at random and decaying exponentially. We find that the particle velocity is maximum for relatively sparse bursts with finite correlation time and non-Gaussian distribution. These occasional kicks, which produce Brownian yet non-Gaussian diffusion, are more efficient for transport and diffusion enhancement of the particle than the incessant kicks of active Ornstein-Uhlenbeck noise.

摘要

众所周知,由于各种活跃过程,活细胞会产生比热涨落大得多的非高斯活跃涨落。理解这些活跃涨落对各种物理化学过程(如分子马达的运输)的影响,是非平衡物理学中的一个基本问题。因此,我们通过实验和数值方法研究了一种活跃布朗棘轮,它由一个胶体粒子组成,处于光学产生的不对称周期势中,由具有有限振幅活跃脉冲的非高斯噪声驱动,每个脉冲随机到达并呈指数衰减。我们发现,对于具有有限相关时间和非高斯分布的相对稀疏的脉冲,粒子速度最大。这些偶尔的推动产生了布朗但非高斯扩散,与活跃的奥恩斯坦 - 乌伦贝克噪声的持续推动相比,对粒子的运输和扩散增强更有效。

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