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方钴矿金属微结构正方形中的低对称性非局域输运

Low-symmetry nonlocal transport in microstructured squares of delafossite metals.

作者信息

McGuinness Philippa H, Zhakina Elina, König Markus, Bachmann Maja D, Putzke Carsten, Moll Philip J W, Khim Seunghyun, Mackenzie Andrew P

机构信息

Physics of Quantum Materials Department, Max Planck Institute for Chemical Physics of Solids, 01187 Dresden, Germany;

Scottish Universities Physics Alliance, School of Physics & Astronomy, University of St. Andrews, St. Andrews KY16 9SS, United Kingdom.

出版信息

Proc Natl Acad Sci U S A. 2021 Nov 23;118(47). doi: 10.1073/pnas.2113185118.

Abstract

Intense work studying the ballistic regime of electron transport in two-dimensional systems based on semiconductors and graphene had been thought to have established most of the key experimental facts of the field. In recent years, however, additional forms of ballistic transport have become accessible in the quasi-two-dimensional delafossite metals, whose Fermi wavelength is a factor of 100 shorter than those typically studied in the previous work and whose Fermi surfaces are nearly hexagonal in shape and therefore strongly faceted. This has some profound consequences for results obtained from the classic ballistic transport experiment of studying bend and Hall resistances in mesoscopic squares fabricated from delafossite single crystals. We observe pronounced anisotropies in bend resistances and even a Hall voltage that is strongly asymmetric in magnetic field. Although some of our observations are nonintuitive at first sight, we show that they can be understood within a nonlocal Landauer-Büttiker analysis tailored to the symmetries of the square/hexagonal geometries of our combined device/Fermi surface system. Signatures of nonlocal transport can be resolved for squares of linear dimension of nearly 100 µm, approximately a factor of 15 larger than the bulk mean free path of the crystal from which the device was fabricated.

摘要

基于半导体和石墨烯的二维系统中电子弹道输运机制的深入研究,被认为已确立了该领域的大部分关键实验事实。然而,近年来,在准二维铜铁矿金属中出现了其他形式的弹道输运,其费米波长比先前研究中通常所研究的短100倍,且其费米面形状近乎六边形,因此具有强烈的晶面。这对于从研究由铜铁矿单晶制成的介观正方形中的弯曲电阻和霍尔电阻的经典弹道输运实验所获得的结果具有一些深远影响。我们观察到弯曲电阻中存在明显的各向异性,甚至在磁场中霍尔电压也强烈不对称。尽管我们的一些观察结果乍一看并不直观,但我们表明,它们可以在针对我们的组合器件/费米面系统的正方形/六边形几何对称性进行定制的非局部朗道尔 - 比蒂克分析中得到理解。对于线性尺寸接近100 µm的正方形,可以分辨出非局部输运的特征,这大约比制造该器件所用晶体的体平均自由程大15倍。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/2b6a/8672864/a284fe81bb8d/pnas.202113185fig01.jpg

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