Department of Oceanography, National Sun Yat-Sen University, Kaohsiung, Taiwan.
The Radiation Monitoring Center, Atomic Energy Council, Kaohsiung, Taiwan.
Sci Rep. 2021 Nov 17;11(1):22467. doi: 10.1038/s41598-021-01895-y.
The release of anthropogenic radiocesium to the North Pacific Ocean (NPO) has occurred in the past 60 years. Factors controlling Cs (half-life, 30.2 year) and Cs (half-life, 2.06 year) activity concentrations in the Kuroshio east of Taiwan and the Taiwan Strait (latitude 20° N-27° N, longitude 116° E-123° E) remain unclear. This study collected seawater samples throughout this region and analyzed Cs and Cs activity concentrations between 2018 and 2019. A principal component analysis (PCA) was performed to analyze the controlling factors of radiocesium. Results of all Cs activity concentrations were below the detection limit (0.5 Bq m). Analyses of water column Cs profiles revealed a primary concentration peak (2.1-2.2 Bq m) at a depth range of 200-400 m (potential density σ 25.3 to 26.1 kg m). The PCA result suggests that this primary peak was related to density layers in the water column. A secondary Cs peak (1.90 Bq m) was observed in the near-surface waters (σ = 18.8 to 21.4 kg m) and was possibly related to upwelling and river-to-sea mixing on the shelf. In the Taiwan Strait, Cs activity concentrations in the near-surface waters were higher in the summer than in the winter. We suggest that upwelling facilitates the vertical transport of Cs at the shelf break of the western NPO.
过去 60 年来,人为放射性铯已释放到北太平洋(NPO)。然而,控制台湾东部黑潮和台湾海峡(北纬 20°N-27°N,东经 116°E-123°E)中 Cs(半衰期 30.2 年)和 Cs(半衰期 2.06 年)活度浓度的因素仍不清楚。本研究于 2018 年至 2019 年在该区域采集海水样本,并分析 Cs 和 Cs 活度浓度。采用主成分分析(PCA)对放射性铯的控制因素进行分析。所有 Cs 活度浓度的结果均低于检测限(0.5 Bq m)。水柱 Cs 浓度剖面分析显示,在 200-400 m 深度范围内存在主要浓度峰值(2.1-2.2 Bq m)(位势密度σ 25.3 至 26.1 kg m)。PCA 结果表明,该主峰与水柱中的密度层有关。在近表层水域(σ=18.8 至 21.4 kg m)观察到次 Cs 峰值(1.90 Bq m),可能与陆架上升流和河海混合有关。在台湾海峡,近表层水域的 Cs 活度浓度夏季高于冬季。我们认为,上升流有利于 NPO 西部陆架边缘的 Cs 垂直输运。