Department of Civil Engineering, Kwame Nkrumah University of Science and Technology, Kumasi, Ghana.
Department of Chemical Engineering, Kwame Nkrumah University of Science and Technology, Kumasi, Ghana.
Sci Rep. 2021 Nov 24;11(1):22830. doi: 10.1038/s41598-021-02276-1.
Non-thermal plasma (NTP) is a promising technology for the improvement of indoor air quality (IAQ) by removing volatile organic compounds (VOCs) through advanced oxidation process (AOP). In this paper, authors developed a laboratory scale dielectric barrier discharge (DBD) reactor which generates atmospheric NTP to study the removal of low-concentration formaldehyde (HCHO), a typical indoor air VOC in the built environment associated with cancer and leukemia, under different processing conditions. Strong ionization NTP was generated between the DBD electrodes by a pulse power zero-voltage switching flyback transformer (ZVS-FBT), which caused ionization of air molecules leading to active species formation to convert HCHO into carbon dioxide (CO) and water vapor (HO). The impact of key electrical and physical processing parameters i.e. discharge power (P), initial concentration (C), flow rate (F), and relative humidity (RH) which affect the formaldehyde removal efficiency (ɳ) were studied to determine optimum conditions. Results show that, the correlation coefficient (R) of removal efficiency dependence on the processing parameters follow the order R (F) = 0.99 > R (RH) = 0.96, > R (C) = 0.94 > R (P) = 0.93. The removal efficiency reached 99% under the optimum conditions of P = 0.6 W, C = 0.1 ppm, F = 0.2 m/h, and RH = 65% with no secondary pollution. The study provided a theoretical and experimental basis for the application of DBD plasma for air purification in the built environment.
非热等离子体(NTP)是一种很有前途的技术,通过先进的氧化过程(AOP)去除挥发性有机化合物(VOCs)来改善室内空气质量(IAQ)。在本文中,作者开发了一种实验室规模的介质阻挡放电(DBD)反应器,该反应器产生大气压 NTP,以研究在不同处理条件下去除低浓度甲醛(HCHO)的情况,HCHO 是一种与癌症和白血病有关的典型室内空气 VOC。通过脉冲功率零电压开关反激变压器(ZVS-FBT)在 DBD 电极之间产生强电离 NTP,这导致空气分子电离,形成活性物质,将 HCHO 转化为二氧化碳(CO)和水蒸气(HO)。研究了影响甲醛去除效率(ɳ)的关键电气和物理处理参数,即放电功率(P)、初始浓度(C)、流速(F)和相对湿度(RH),以确定最佳条件。结果表明,去除效率对处理参数的相关性系数(R)的顺序为 R(F)=0.99> R(RH)=0.96> R(C)=0.94> R(P)=0.93。在最佳条件下,即 P=0.6 W、C=0.1 ppm、F=0.2 m/h 和 RH=65%时,去除效率达到 99%,且无二次污染。该研究为 DBD 等离子体在建筑环境中的空气净化应用提供了理论和实验基础。