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沿海土壤和沉积物中多环芳烃(PAHs)的污染与修复综述

Review on the contamination and remediation of polycyclic aromatic hydrocarbons (PAHs) in coastal soil and sediments.

作者信息

Dai Chaomeng, Han Yueming, Duan Yanping, Lai Xiaoying, Fu Rongbing, Liu Shuguang, Leong Kah Hon, Tu Yaojen, Zhou Lang

机构信息

College of Civil Engineering, Tongji University, 1239 Siping Road, Shanghai, 200092, PR China.

Institute of Urban Studies, School of Environmental and Geographical Sciences, Shanghai Normal University, 100 Guilin Rd., Shanghai, 200234, PR China; Yangtze River Delta Urban Wetland Ecosystem National Field Observation and Research Station, Shanghai, 200234, China.

出版信息

Environ Res. 2022 Apr 1;205:112423. doi: 10.1016/j.envres.2021.112423. Epub 2021 Nov 24.

Abstract

The rapid economic and population growth in coastal areas is causing increasingly serious polycyclic aromatic hydrocarbons (PAHs) pollution in these regions. This review compared the PAHs pollution characteristics of different coastal areas, including industrial zones, commercial ports, touristic cities, aquacultural & agricultural areas, oil & gas exploitation areas and megacities. Currently there are various treatment methods to remediate soils and sediments contaminated with PAHs. However, it is necessary to provide a comprehensive overview of all the available remediation technologies up to date, so appropriate technologies can be selected to remediate PAHs pollution. In view of that, we analyzed the characteristics of the remediation mechanism, summarized the remediation methods for soil or sediments in coastal areas, which were physical repair, chemical oxidation, bioremediation and integrated approaches. Besides, this review also reported the development of new multi-functional green and sustainable systems, namely, micro-nano bubble (MNB), biochar, reversible surfactants and peracetic acid. While physical repair, expensive but efficient, was regarded as a suitable method for the PAHs remediation in coastal areas because of land shortage, integrated approaches would produce better results. The ultimate aim of the review was to ensure the successful restructuring of PAHs contaminated soil and sediments in coastal areas. Due to the environment heterogeneity, PAHs pollution in coastal areas remains as a daunting challenge. Therefore, new and suitable technologies are still needed to address the environmental issue.

摘要

沿海地区快速的经济增长和人口增长正导致这些地区多环芳烃(PAHs)污染日益严重。本综述比较了不同沿海地区的PAHs污染特征,包括工业区、商业港口、旅游城市、水产养殖和农业区、油气开采区以及大城市。目前有多种处理方法可用于修复受PAHs污染的土壤和沉积物。然而,有必要对目前所有可用的修复技术进行全面概述,以便能够选择合适的技术来修复PAHs污染。鉴于此,我们分析了修复机制的特点,总结了沿海地区土壤或沉积物的修复方法,包括物理修复、化学氧化、生物修复和综合方法。此外,本综述还报道了新型多功能绿色可持续系统的发展,即微纳米气泡(MNB)、生物炭、可逆表面活性剂和过氧乙酸。虽然物理修复成本高昂但效率高,由于土地短缺,被认为是沿海地区PAHs修复的合适方法,但综合方法可能会产生更好的效果。本综述的最终目的是确保成功修复沿海地区受PAHs污染的土壤和沉积物。由于环境的异质性,沿海地区的PAHs污染仍然是一项艰巨的挑战。因此,仍需要新的合适技术来解决这一环境问题。

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