Functional Materials and Microsystems Research Group and the Micro Nano Research Facility, RMIT University, Melbourne, Victoria 3001, Australia.
Department of Biomedical Engineering, University of Arizona, Tucson, Arizona 85721, United States.
ACS Sens. 2022 Jan 28;7(1):82-88. doi: 10.1021/acssensors.1c01633. Epub 2021 Dec 8.
Nicotine, an addictive substance in tobacco products and electronic cigarettes (e-cigs), is recognized for increasing the risk of cardiovascular and respiratory disorders. Careful real-time monitoring of nicotine exposure is critical in alleviating the potential health impacts of not just smokers but also those exposed to second-hand and third-hand smoke. Monitoring of nicotine requires suitable sensing material to detect nicotine selectively and testing under free-living conditions in the standard environment. Here, we experimentally demonstrate a vanadium dioxide (VO)-based nicotine sensor and explain its conductometric mechanisms with compositional analysis and density functional theory (DFT) calculations. For real-time monitoring of nicotine vapor from e-cigarettes in the air, the sensor is integrated with an epidermal near-field communication (NFC) interface that enables battery-free operation and data transmission to smart electronic devices to record and store sensor data. Collectively, the technique of sensor development and integration expands the use of wearable electronics for real-time monitoring of hazardous elements in the environment and biosignals wirelessly.
尼古丁是烟草制品和电子烟(e-cigs)中的一种成瘾物质,已被证实会增加心血管和呼吸系统疾病的风险。在减轻不仅是吸烟者,还有那些接触二手烟和三手烟的人潜在健康影响方面,对尼古丁暴露进行仔细的实时监测至关重要。监测尼古丁需要合适的传感材料来选择性地检测尼古丁,并在标准环境下的自由生活条件下进行测试。在这里,我们通过实验展示了一种基于二氧化钒(VO)的尼古丁传感器,并通过组成分析和密度泛函理论(DFT)计算解释了其传导机制。为了实时监测空气中电子烟产生的尼古丁蒸气,该传感器与表皮近场通信(NFC)接口集成,实现了电池供电操作和数据传输到智能电子设备,以记录和存储传感器数据。总的来说,传感器开发和集成技术扩展了可穿戴电子设备在环境中有害物质和生物信号的实时无线监测中的应用。