College of Energy and Mechanical Engineering, Shanghai University of Electric Power, Shanghai, China; Shanghai Engineering Research Center of Power Generation Environment Protection, Shanghai, China.
College of Energy and Mechanical Engineering, Shanghai University of Electric Power, Shanghai, China.
Chemosphere. 2022 May;295:133834. doi: 10.1016/j.chemosphere.2022.133834. Epub 2022 Feb 3.
Photocatalytic degradation technology is regarded as a promising technology for dye-contained wastewater treatment due to its superior efficiency and recycling. The key to the implementation of photocatalytic degradation technology is the selection of sunlight-active photocatalyst. Graphitic carbon nitride (g-CN) photocatalyst has been put into a lot of research in the field of organic pollutant degradation because of its low cost, suitable electronic structure and high chemical stability. In this perspective review, we comprehensively discuss the recent advance of photocatalytic dyes degradation over g-CN-based materials. The properties, structure and preparation methods of g-CN are briefly introduced. Furthermore, the progress in improving the degradation efficiency of g-CN-based photocatalyst is highlighted in the article. The possible pathways and different active species for dyes decomposition are also summarized. We expect this review can provide instructive application of g-CN-based catalysts for environmental remediation.
光催化降解技术因其高效、可回收等优点,被认为是一种很有前途的含染料废水处理技术。实施光催化降解技术的关键在于选择太阳光活性光催化剂。石墨相氮化碳(g-CN)光催化剂由于其低成本、合适的电子结构和高化学稳定性,在有机污染物降解领域得到了大量研究。在本综述中,我们全面讨论了 g-CN 基材料在光催化染料降解方面的最新进展。简要介绍了 g-CN 的性质、结构和制备方法。此外,文章还重点介绍了提高 g-CN 基光催化剂降解效率的进展。还总结了染料分解的可能途径和不同的活性物质。我们希望本综述能为 g-CN 基催化剂在环境修复中的应用提供有指导意义的参考。