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关于基于 g-CN 的光催化剂在去除有机污染物方面的高级可重复利用性的综合综述。

Comprehensive review on advanced reusability of g-CN based photocatalysts for the removal of organic pollutants.

机构信息

Process Intensification Laboratory, Department of Chemical Engineering, National Institute of Technology Rourkela, Rourkela, Odisha, 769 008, India.

Process Intensification Laboratory, Department of Chemical Engineering, National Institute of Technology Rourkela, Rourkela, Odisha, 769 008, India.

出版信息

Chemosphere. 2022 Jun;297:134190. doi: 10.1016/j.chemosphere.2022.134190. Epub 2022 Mar 3.

Abstract

Graphitic carbon nitride (g-CN) has attained significant research attention in energy and environmental remediation due to its excellent electronic structure, greater physical and chemical properties, and abundance. However, graphitic carbon nitride faces severe problems because of its high recombination rate and higher mass loss of the catalyst during recovery operations. This review emphasizes the methods to overcome the difficulties associated with recovery and reusability of the g-CN based photocatalyst towards the redemption of pollutants present in wastewater. Different strategies like magnetic g-CN based photocatalysts, immobilized photocatalytic systems, and photocatalytic membranes and their usage in photocatalytic applications are well described. Different preparation strategies of the graphic carbon nitride-based composites are elucidated. The key challenges and future perspectives of adopting these methods for photocatalytic applications are also mentioned.

摘要

石墨相氮化碳(g-CN)因其优异的电子结构、更好的物理化学性质和丰富的储量,在能源和环境修复领域引起了广泛的关注。然而,石墨相氮化碳面临着严重的问题,因为其高复合率和催化剂在回收操作过程中的更高质量损失。本综述强调了克服基于 g-CN 的光催化剂回收和再利用困难的方法,以回收废水中存在的污染物。详细描述了不同的策略,如基于磁性 g-CN 的光催化剂、固定化光催化系统、光催化膜及其在光催化应用中的应用。阐述了基于图形碳氮化物的复合材料的不同制备策略。还提到了采用这些方法进行光催化应用的关键挑战和未来展望。

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