Jang Hoyoung, Song Sanghoon, Kihara Takumi, Liu Yijin, Lee Sang-Jun, Park Sang-Youn, Kim Minseok, Kim Hyeong-Do, Coslovich Giacomo, Nakata Suguru, Kubota Yuya, Inoue Ichiro, Tamasaku Kenji, Yabashi Makina, Lee Heemin, Song Changyong, Nojiri Hiroyuki, Keimer Bernhard, Kao Chi-Chang, Lee Jun-Sik
PAL-XFEL, Pohang Accelerator Laboratory, Pohang, Gyeongbuk 37673, Republic of Korea.
Photon Science Center, Pohang University of Science and Technology, Pohang, Gyeongbuk 37673, Republic of Korea.
Sci Adv. 2022 Feb 11;8(6):eabk0832. doi: 10.1126/sciadv.abk0832. Epub 2022 Feb 9.
The normal state of high- cuprates has been considered one of the essential topics in high-temperature superconductivity research. However, compared to the high magnetic field study of it, understanding a photoinduced normal state remains elusive. Here, we explore a photoinduced normal state of YBaCuO through a charge density wave (CDW) with time-resolved resonant soft x-ray scattering, as well as a high magnetic field x-ray scattering. In the nonequilibrium state where people predict a quenched superconducting state based on the previous optical spectroscopies, we experimentally observed a similar analogy to the competition between superconductivity and CDW shown in the equilibrium state. We further observe that the broken pairing states in the superconducting CuO plane via the optical pump lead to nucleation of three-dimensional CDW precursor correlation. Ultimately, these findings provide a critical clue that the characteristics of the photoinduced normal state show a solid resemblance to those under magnetic fields in equilibrium conditions.
高铜酸盐的正常态一直被认为是高温超导研究中的核心课题之一。然而,与对其进行的高磁场研究相比,对光致正常态的理解仍然不够清晰。在此,我们通过时间分辨共振软X射线散射以及高磁场X射线散射,利用电荷密度波(CDW)来探索YBaCuO的光致正常态。在基于先前光谱学人们预测会出现猝灭超导态的非平衡态中,我们通过实验观察到了与平衡态中超导性和CDW之间竞争的类似情况。我们进一步观察到,通过光泵浦导致超导CuO平面中的配对态破裂,从而引发三维CDW前驱体关联的成核。最终,这些发现提供了一个关键线索,即光致正常态的特征与平衡条件下磁场中的特征极为相似。