Max Planck Institute for Solid State Research, Heisenbergstraße 1, D-70569 Stuttgart, Germany.
European Synchrotron Radiation Facility (ESRF), BP 220, F-38043 Grenoble Cedex, France.
Science. 2018 Nov 30;362(6418):1040-1044. doi: 10.1126/science.aat4708.
Cuprates exhibit antiferromagnetic, charge density wave (CDW), and high-temperature superconducting ground states that can be tuned by means of doping and external magnetic fields. However, disorder generated by these tuning methods complicates the interpretation of such experiments. Here, we report a high-resolution inelastic x-ray scattering study of the high-temperature superconductor YBaCuO under uniaxial stress, and we show that a three-dimensional long-range-ordered CDW state can be induced through pressure along the axis, in the absence of magnetic fields. A pronounced softening of an optical phonon mode is associated with the CDW transition. The amplitude of the CDW is suppressed below the superconducting transition temperature, indicating competition with superconductivity. The results provide insights into the normal-state properties of cuprates and illustrate the potential of uniaxial-pressure control of competing orders in quantum materials.
铜酸盐表现出反铁磁、电荷密度波(CDW)和高温超导基态,这些状态可以通过掺杂和外磁场来调节。然而,这些调节方法产生的无序使得这些实验的解释变得复杂。在这里,我们报告了在单轴压力下高温超导体 YBaCuO 的高分辨率非弹性 X 射线散射研究,结果表明,在没有磁场的情况下,沿[001]轴施加压力可以诱导出三维长程有序的 CDW 态。一个光学声子模式的明显软化与 CDW 转变相关。在超导转变温度以下,CDW 的幅度被抑制,表明与超导性竞争。这些结果提供了对铜酸盐正常态性质的深入了解,并说明了在量子材料中通过单轴压力控制竞争序的潜力。