Boschini F, da Silva Neto E H, Razzoli E, Zonno M, Peli S, Day R P, Michiardi M, Schneider M, Zwartsenberg B, Nigge P, Zhong R D, Schneeloch J, Gu G D, Zhdanovich S, Mills A K, Levy G, Jones D J, Giannetti C, Damascelli A
Department of Physics & Astronomy, University of British Columbia, Vancouver, BC, Canada.
Quantum Matter Institute, University of British Columbia, Vancouver, BC, Canada.
Nat Mater. 2018 May;17(5):416-420. doi: 10.1038/s41563-018-0045-1. Epub 2018 Apr 2.
The possibility of driving phase transitions in low-density condensates through the loss of phase coherence alone has far-reaching implications for the study of quantum phases of matter. This has inspired the development of tools to control and explore the collective properties of condensate phases via phase fluctuations. Electrically gated oxide interfaces, ultracold Fermi atoms and cuprate superconductors, which are characterized by an intrinsically small phase stiffness, are paradigmatic examples where these tools are having a dramatic impact. Here we use light pulses shorter than the internal thermalization time to drive and probe the phase fragility of the BiSrCaCuO cuprate superconductor, completely melting the superconducting condensate without affecting the pairing strength. The resulting ultrafast dynamics of phase fluctuations and charge excitations are captured and disentangled by time-resolved photoemission spectroscopy. This work demonstrates the dominant role of phase coherence in the superconductor-to-normal state phase transition and offers a benchmark for non-equilibrium spectroscopic investigations of the cuprate phase diagram.
仅通过相位相干性的丧失来驱动低密度凝聚态中的相变,这一可能性对量子物质相的研究具有深远影响。这激发了通过相位涨落来控制和探索凝聚态相集体性质的工具的发展。以固有小相位刚度为特征的电门控氧化物界面、超冷费米原子和铜酸盐超导体,是这些工具产生巨大影响的典型例子。在这里,我们使用比内部热化时间短的光脉冲来驱动和探测BiSrCaCuO铜酸盐超导体的相位脆弱性,完全熔化超导凝聚态而不影响配对强度。时间分辨光电子能谱捕捉并解开了由此产生的相位涨落和电荷激发的超快动力学。这项工作证明了相位相干性在超导体到正常态相变中的主导作用,并为铜酸盐相图的非平衡光谱研究提供了一个基准。