Yuan Jie, Chen Qihong, Jiang Kun, Feng Zhongpei, Lin Zefeng, Yu Heshan, He Ge, Zhang Jinsong, Jiang Xingyu, Zhang Xu, Shi Yujun, Zhang Yanmin, Qin Mingyang, Cheng Zhi Gang, Tamura Nobumichi, Yang Yi-Feng, Xiang Tao, Hu Jiangping, Takeuchi Ichiro, Jin Kui, Zhao Zhongxian
Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing, China.
Key Laboratory of Vacuum Physics, School of Physical Sciences, University of Chinese Academy of Sciences, Beijing, China.
Nature. 2022 Feb;602(7897):431-436. doi: 10.1038/s41586-021-04305-5. Epub 2022 Feb 16.
Marked evolution of properties with minute changes in the doping level is a hallmark of the complex chemistry that governs copper oxide superconductivity as manifested in the celebrated superconducting domes and quantum criticality taking place at precise compositions. The strange-metal state, in which the resistivity varies linearly with temperature, has emerged as a central feature in the normal state of copper oxide superconductors. The ubiquity of this behaviour signals an intimate link between the scattering mechanism and superconductivity. However, a clear quantitative picture of the correlation has been lacking. Here we report the observation of precise quantitative scaling laws among the superconducting transition temperature (T), the linear-in-T scattering coefficient (A) and the doping level (x) in electron-doped copper oxide LaCeCuO (LCCO). High-resolution characterization of epitaxial composition-spread films, which encompass the entire overdoped range of LCCO, has enabled us to systematically map its structural and transport properties with unprecedented accuracy and with increments of Δx = 0.0015. We have uncovered the relations T ~ (x - x) ~ (A), where x is the critical doping in which superconductivity disappears and A is the coefficient of the linear resistivity per CuO plane. The striking similarity of the T versus A relation among copper oxides, iron-based and organic superconductors may be an indication of a common mechanism of the strange-metal behaviour and unconventional superconductivity in these systems.
掺杂水平的微小变化会导致性质发生显著演变,这是复杂化学的一个标志,这种复杂化学支配着氧化铜超导性,体现在著名的超导穹顶以及在精确成分下发生的量子临界性中。电阻率随温度线性变化的奇异金属态,已成为氧化铜超导体正常态的一个核心特征。这种行为的普遍性表明散射机制与超导性之间存在紧密联系。然而,一直缺乏这种关联的清晰定量描述。在此,我们报告在电子掺杂的氧化铜LaCeCuO(LCCO)中,观察到超导转变温度(T)、T线性散射系数(A)和掺杂水平(x)之间精确的定量标度律。对涵盖LCCO整个过掺杂范围的外延成分渐变薄膜进行高分辨率表征,使我们能够以前所未有的精度、以Δx = 0.0015的增量系统地绘制其结构和输运性质。我们发现了关系T ~ (x - x) ~ (A),其中x是超导性消失时的临界掺杂,A是每个CuO平面的线性电阻率系数。铜氧化物、铁基和有机超导体中T与A关系的显著相似性,可能表明这些系统中奇异金属行为和非常规超导性存在共同机制。