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通过表面晶格共振与法布里-珀罗共振的强耦合实现金属纳米棒周围大体积区域的显著近场增强。

Significant Near-Field Enhancement over Large Volumes around Metal Nanorods via Strong Coupling of Surface Lattice Resonances and Fabry-Pérot Resonance.

作者信息

Shi Yunjie, Dong Yuming, Sun Degui, Li Guangyuan

机构信息

Schools of Science, Changchun University of Science and Technology, 7089 Weixing Road, Changchun 130022, China.

CAS Key Laboratory of Human-Machine Intelligence-Synergy Systems, Shenzhen Institute of Advanced Technology, Chinese Academy of Sciences, Shenzhen 518055, China.

出版信息

Materials (Basel). 2022 Feb 18;15(4):1523. doi: 10.3390/ma15041523.

Abstract

Metal nanoparticles supporting plasmons are widely used to enhance electromagnetic fields, resulting in strong light-matter interactions at the nanoscale in a diverse range of applications. Recently, it has been shown that when metal nanorods are periodically arranged with proper lattice periods, surface lattice resonances (SLRs) can be excited and near fields can be greatly enhanced over extended volumes. In this work, we report significant near field enhancement over even larger volumes by placing the metal nanorod array within a Fabry-Pérot (F-P) microcavity. Simulation results show that by taking advantage of strong coupling between the SLR and the photonic F-P resonances, the electric field intensity of the bonding split mode can be enhanced by up to 1935 times, which is about three times of the enhancement of the SLR, and the greatly enhanced field can extend over most of the F-P microcavity. We further show that the F-P resonances of both odd and even orders can strongly couple to the SLR by varying the nanorods position from the middle of the microcavity. We expect that the proposed plasmonic-photonic coupling system will find promising applications in nanolasers, nonlinear optics and sensing.

摘要

支持表面等离激元的金属纳米粒子被广泛用于增强电磁场,从而在各种应用的纳米尺度上产生强烈的光与物质相互作用。最近,研究表明,当金属纳米棒以适当的晶格周期周期性排列时,可以激发表面晶格共振(SLR),并且在扩展体积内近场可以得到极大增强。在这项工作中,我们报告了通过将金属纳米棒阵列置于法布里 - 珀罗(F - P)微腔内,在甚至更大的体积上实现了显著的近场增强。模拟结果表明,利用SLR与光子F - P共振之间的强耦合,键合分裂模式的电场强度可以增强高达1935倍,这约为SLR增强的三倍,并且大大增强的场可以扩展到大部分F - P微腔。我们进一步表明,通过改变纳米棒在微腔中间的位置,奇数阶和偶数阶的F - P共振都可以与SLR强烈耦合。我们预计所提出的等离激元 - 光子耦合系统将在纳米激光器、非线性光学和传感领域找到有前景的应用。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/184e/8876971/b15ce2a428aa/materials-15-01523-g001.jpg

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