Lu Lu, Zhang Bo, Ou Han, Li Bowen, Zhou Kun, Song Jinlin, Luo Zixue, Cheng Qiang
State Key Laboratory of Coal Combustion, School of Energy and Power Engineering, Huazhong University of Science and Technology, Wuhan, Hubei, 430074, China.
School of Electrical and Information Engineering, Wuhan Institute of Technology, Wuhan, Hubei, 430025, China.
Small. 2022 May;18(19):e2108032. doi: 10.1002/smll.202108032. Epub 2022 Mar 11.
Near-field radiative heat transfer (NFRHT) can exceed the blackbody radiation limit owing to the coupled evanescent waves, implying a significant potential for energy conversion and thermal management. Coupled surface plasmon polaritons (SPPs) and hyperbolic phonon polaritons (HPPs) with small ohmic losses enable a long propagation wavelength that is essential in NFRHT. However, so far, there still lacks knowledge about the experimental investigation of the coupling of SPPs and HPPs in terms of NFRHT. In this study, the NFRHT between graphene/hexagonal boron nitride (hBN) systems that can be readily transferred onto various substrates, with a gap space of ≈400 nm is measured. NFRHT enhancements in the order of three and six times higher than the blackbody limit for graphene/hBN heterostructures and graphene/hBN/graphene multilayers, respectively are demonstrated. In addition, the largest ever radiative heat flux using graphene/hBN/graphene multilayers under similar gap space of 400 nm is obtained. Consequently, analyzing the photon tunneling modes reveal that these phenomena are consequences of coupled SPPs of graphene and HPPs of hBN.
近场辐射热传递(NFRHT)由于耦合倏逝波能够超过黑体辐射极限,这意味着在能量转换和热管理方面具有巨大潜力。具有小欧姆损耗的耦合表面等离激元极化激元(SPPs)和双曲声子极化激元(HPPs)能够实现长传播波长,这在近场辐射热传递中至关重要。然而,到目前为止,在近场辐射热传递方面,关于表面等离激元极化激元和双曲声子极化激元耦合的实验研究仍然缺乏相关知识。在本研究中,测量了石墨烯/六方氮化硼(hBN)系统之间的近场辐射热传递,该系统可以很容易地转移到各种衬底上,间隙空间约为400纳米。结果表明,石墨烯/hBN异质结构和石墨烯/hBN/石墨烯多层结构的近场辐射热传递增强分别比黑体极限高出三倍和六倍。此外,在400纳米的相似间隙空间下,使用石墨烯/hBN/石墨烯多层结构获得了有史以来最大的辐射热通量。因此,对光子隧穿模式的分析表明,这些现象是石墨烯的表面等离激元极化激元和六方氮化硼的双曲声子极化激元耦合的结果。