Li Jingbo, Ma Wanli, Jiang Lin, Yao Niangjuan, Deng Jie, Qiu Qinxi, Shi Yi, Zhou Wei, Huang Zhiming
State Key Laboratory of Infrared Physics, Shanghai Institute of Technical Physics, Chinese Academy of Sciences, 500 Yu Tian Road, Shanghai 200083, P. R. China.
University of Chinese Academy of Sciences, 19 Yu Quan Road, Beijing 100049, P. R. China.
ACS Appl Mater Interfaces. 2022 Mar 30;14(12):14331-14341. doi: 10.1021/acsami.2c00175. Epub 2022 Mar 15.
Photoelectric detection is developing rapidly from ultraviolet to infrared band. However, terahertz (THz) photodetection approaches is constrained by the bandgap, dark current, and absorption ability. In this work, room-temperature photoelectric detection is extended to the THz range implemented in a planar metal-NbSe-metal structure based on an electromagnetic induced well (EIW) theory, exhibiting an excellent broadband responsivity of 5.2 × 10 V W at 0.027 THz, 7.8 × 10 V W at 0.173 THz, and 9.6 × 10 V W at 0.259 THz. Simultaneously, the NbSe photoelectric detector (PD) with ultrafast response speed (∼610 ns) and ultralow equivalent noise power (4.6 × 10 W Hz) in the THz region is realized, enabling high-resolution imaging. The figure of merit (FOM) characterizing the detection performance of the device is 2 orders of magnitude superior to that of the reported THz PDs based 2D materials. Furthermore, the THz response speed is 2 orders of magnitude faster than that of the visible due to the different response mechanisms of the device. Our results exhibit promising potential to achieve highly sensitive and ultrafast photoelectric detection.
光电探测正从紫外波段迅速发展到红外波段。然而,太赫兹(THz)光电探测方法受到带隙、暗电流和吸收能力的限制。在这项工作中,基于电磁感应阱(EIW)理论,将室温光电探测扩展到在平面金属 - 铌硒化物 - 金属结构中实现的太赫兹范围,在0.027太赫兹时表现出5.2×10 V/W的优异宽带响应率,在0.173太赫兹时为7.8×10 V/W,在0.259太赫兹时为9.6×10 V/W。同时,实现了在太赫兹区域具有超快响应速度(约610纳秒)和超低等效噪声功率(4.6×10 W/Hz)的铌硒化物光电探测器(PD),能够进行高分辨率成像。表征该器件探测性能的品质因数(FOM)比报道的基于二维材料的太赫兹PDs高出2个数量级。此外,由于器件的响应机制不同,太赫兹响应速度比可见光快2个数量级。我们的结果显示出实现高灵敏度和超快光电探测的巨大潜力。