Shen Pingchuan, Liu Hao, Zhuang Zeyan, Zeng Jiajie, Zhao Zujin, Tang Ben Zhong
State Key Laboratory of Luminescent Materials and Devices, Guangdong Provincial Key Laboratory of Luminescence from Molecular Aggregates, South China University of Technology, Guangzhou, 510640, China.
Shenzhen Institute of Aggregate Science and Technology, School of Science and Engineering, The Chinese University of Hong Kong, Shenzhen, Guangdong, 518172, China.
Adv Sci (Weinh). 2022 May;9(15):e2200374. doi: 10.1002/advs.202200374. Epub 2022 Mar 24.
Thermally stable electron transport (ET) materials with high electron mobility and high triplet state energy level are highly desired for the fabrication of efficient and stable organic light-emitting diodes (OLEDs). Herein, a new design strategy of constructing through-space conjugated folded configuration is proposed to explore robust ET materials, opposite to the widely used planar configuration. By bonding two quinolines to the 9,10-positions of phenanthrene, two novel folded molecules with high thermal and morphological stabilities and high triplet state energy levels (>2.7 eV) are created. These folded molecules possess excellent ET ability with electron mobilities of three orders of magnitude higher than those of linear and planar counterparts. Theoretical calculation and crystallography analysis demonstrate the through-space conjugated folded configuration has not only reduced reorganization energy but also enlarged charge transfer integral at various dimensions, bringing about efficient multi-dimensional ET, independent of molecular orientation. By adopting the folded molecule as ET layers, OLEDs with no matter delayed fluorescence or phosphorescence emitters can achieve high external quantum efficiencies and long operational lifetimes simultaneously. This work paves a new avenue towards robust ET materials to improve efficiency and stability of OLEDs.
对于高效且稳定的有机发光二极管(OLED)的制造而言,非常需要具有高电子迁移率和高三重态能级的热稳定电子传输(ET)材料。在此,提出了一种构建空间共轭折叠构型的新设计策略,以探索坚固的ET材料,这与广泛使用的平面构型相反。通过将两个喹啉连接到菲的9,10位,制备出了两种具有高热稳定性和形态稳定性以及高三重态能级(>2.7 eV)的新型折叠分子。这些折叠分子具有出色的ET能力,其电子迁移率比线性和平面对应物高三个数量级。理论计算和晶体学分析表明,空间共轭折叠构型不仅降低了重组能,而且在各个维度上扩大了电荷转移积分,实现了高效的多维ET,且与分子取向无关。通过采用折叠分子作为ET层,无论使用延迟荧光还是磷光发射体的OLED都能同时实现高外部量子效率和长工作寿命。这项工作为开发坚固的ET材料以提高OLED的效率和稳定性开辟了一条新途径。