Ren Z X, Vretenar D, Nikšić T, Zhao P W, Zhao J, Meng J
State Key Laboratory of Nuclear Physics and Technology, School of Physics, Peking University, Beijing 100871, China.
Physics Department, Faculty of Science, University of Zagreb, 10000 Zagreb, Croatia.
Phys Rev Lett. 2022 Apr 29;128(17):172501. doi: 10.1103/PhysRevLett.128.172501.
In the exothermic process of fission decay, an atomic nucleus splits into two or more independent fragments. Several aspects of nuclear fission are not properly understood, in particular the formation of the neck between the nascent fragments, and the subsequent mechanism of scission into two or more independent fragments. Using an implementation of time-dependent density functional theory, based on a relativistic energy density functional and including pairing correlations, we analyze the final phase of the process of induced fission of ^{240}Pu, and show that the timescale of neck formation coincides with the assembly of two α-like clusters. Because of its much larger binding energy, the dynamical synthesis of ^{4}He in the neck predominates over other light clusters, e.g., ^{3}H and ^{6}He. At the instant of scission the neck ruptures exactly between the two α-like clusters, which separate because of the Coulomb repulsion and are eventually absorbed by the two emerging fragments. The mechanism of light charged clusters formation at scission could also be linked to ternary fission.
在裂变衰变的放热过程中,一个原子核分裂成两个或更多独立的碎片。核裂变的几个方面尚未得到充分理解,特别是新生碎片之间颈部的形成以及随后分裂成两个或更多独立碎片的机制。我们使用基于相对论能量密度泛函并包含配对关联的含时密度泛函理论的一种实现方式,分析了(^{240}Pu)诱发裂变过程的最后阶段,并表明颈部形成的时间尺度与两个类α簇的组装相吻合。由于其大得多的结合能,颈部中(^{4}He)的动态合成比其他轻簇(例如(^{3}H)和(^{6}He))占主导。在裂变瞬间,颈部恰好在两个类α簇之间断裂,这两个簇由于库仑排斥而分离,并最终被两个新生碎片吸收。裂变时轻带电簇形成的机制也可能与三元裂变有关。