Liu Yijie, Guo Yujun, Zhang Xueqin, Gao Guoqiang, Shi Chaoqun, Huang Guizao, Li Pengli, Kang Qi, Huang Xingyi, Wu Guangning
College of Electrical Engineering, Southwest Jiaotong University, Chengdu, 611756 China.
Department of Polymer Science and Engineering, Shanghai Key Laboratory of Electrical Insulation and Thermal Ageing, State Key laboratory of Metal Matrix Composites, Shanghai Jiaotong University, Shanghai, 200240 China.
Nano Res. 2022;15(5):4732-4738. doi: 10.1007/s12274-022-4093-0. Epub 2022 Feb 8.
Self-cleaning is the key factor that makes superhydrophobic nanostructured materials have wide applications. The self-cleaning effect, however, strongly depends on formations and movement of water droplets on superhydrophobic nanostructured surfaces, which is greatly restricted at low humidity (< 7.6 g·kg). Therefore, we propose a self-cleaning method at low humidity in which the pollution is electro-aggregated and driven in the electric field to achieve the aggregation and cleaning large areas. The cleaning efficiency of this method is much higher than that of water droplet roll-off, and will not produce "pollution bands". A simplified numerical model describing pollution movements is presented. Simulation results are consistent with experimental results. The proposed method realizes the self-cleaning of superhydrophobic nanostructured surfaces above dew point curve for the first time, which extends applications of superhydrophobic nanostructured materials in low humidity, and is expected to solve self-cleaning problems of outdoor objects in low humidity areas (< 5.0 g·kg).
Supplementary material (experimental procedures, computational details, modeling process, supplementary figures, tables, and videos) is available in the online version of this article at 10.1007/s12274-022-4093-0.
自清洁是使超疏水纳米结构材料具有广泛应用的关键因素。然而,自清洁效果很大程度上取决于超疏水纳米结构表面上水滴的形成和移动,在低湿度(<7.6 g·kg)条件下这受到极大限制。因此,我们提出一种在低湿度下的自清洁方法,其中污染物在电场中被电聚集并驱动,以实现大面积的聚集和清洁。该方法的清洁效率远高于水滴滚落法,且不会产生“污染带”。提出了一个描述污染物移动的简化数值模型。模拟结果与实验结果一致。所提出的方法首次实现了超疏水纳米结构表面在露点曲线以上的自清洁,拓展了超疏水纳米结构材料在低湿度环境下的应用,有望解决低湿度地区(<5.0 g·kg)户外物体的自清洁问题。
补充材料(实验步骤、计算细节、建模过程、补充图、表和视频)可在本文的在线版本中获取,链接为10.1007/s12274-022-4093-0。