School of Chemistry, Sun Yat-sen University, Guangzhou, 510275, China.
Instrumental Analysis and Research Center (IARC), Sun Yat-Sen University, Guangzhou, 510275, China.
Angew Chem Int Ed Engl. 2022 Aug 1;61(31):e202206749. doi: 10.1002/anie.202206749. Epub 2022 Jun 21.
The escalating contamination by per- and polyfluoroalkyl substances (PFAS) has become an urgent issue in recent years, and the structural diversity of PFAS is the major challenge for effective pollution control. Herein, we take the intrinsic advantages of squaramide and prepare a new two-dimensional covalent organic framework (FSQ-1) that exhibits broad-spectrum PFAS affinity. The tailor-made linker forges hydrogen-bond donors, hydrogen-bond acceptors, and fluorophilic segments into one framework. The obtained material exhibits multipoint and multitype affinity to PFAS with different structures, by which high-efficient and broad-spectrum removal of various PFAS can be simultaneously achieved. Notably, the thermodynamic profiles provided by isothermal titration calorimetry (ITC) experiments further illustrate the underlying mechanism of the broad-spectrum affinity. FSQ-1 can also be applied for efficient PFAS extraction in trace-level PFAS analysis.
近年来,全氟和多氟烷基物质 (PFAS) 的污染不断加剧,已成为一个紧迫的问题,而 PFAS 的结构多样性是有效污染控制的主要挑战。在本文中,我们利用酰亚胺的固有优势,制备了一种新的二维共价有机框架 (FSQ-1),该框架对广谱 PFAS 具有亲和力。定制的连接基将氢键供体、氢键受体和亲氟片段结合到一个框架中。所得到的材料对具有不同结构的各种 PFAS 表现出多点和多类型的亲和力,从而可以同时实现高效和广谱去除各种 PFAS。值得注意的是,等温滴定微量热法 (ITC) 实验提供的热力学曲线进一步说明了广谱亲和力的潜在机制。FSQ-1 还可以用于痕量水平 PFAS 分析中 PFAS 的高效提取。