Orgiani Pasquale, Galdi Alice, Schlom Darrell G, Maritato Luigi
CNR-IOM, TASC Laboratory in Area Science Park, 34139 Trieste, Italy.
Dipartimento di Ingegneria Industriale, Università degli Studi di Salerno, 84084 Fisciano, Italy.
Nanomaterials (Basel). 2022 May 17;12(10):1709. doi: 10.3390/nano12101709.
Transport properties of electron-doped cuprate Sr1-xLaxCuO2 thin films have been investigated as a function of doping. In particular, optimal- and over-doped samples were obtained by tuning the Sr:La stoichiometric ratio. Optimal-doped samples show a non-Fermi liquid behavior characterized by linear dependence of the resistivity from room temperature down to intermediate temperature (about 150-170 K). However, by approaching temperatures in the superconducting transition, a Fermi-liquid behavior-characterized by a T2-scaling law-was observed. Once established, the transition from a linear- to a quadratic-T2 behavior was successfully traced back in over-doped samples, even occurring at lower temperatures. In addition, the over-doped samples show a crossover to a linear- to a logarithmic dependence at high temperatures compatible with anti-ferromagnetic spin fluctuations dominating the normal state properties of electron-doped cuprates.
研究了电子掺杂铜酸盐Sr1-xLaxCuO2薄膜的输运性质随掺杂的变化。特别是,通过调整Sr:La化学计量比获得了最佳掺杂和过掺杂样品。最佳掺杂样品表现出非费米液体行为,其特征是电阻率从室温到中间温度(约150 - 170K)呈线性依赖关系。然而,在接近超导转变温度时,观察到了以T2标度律为特征的费米液体行为。一旦确定,在过掺杂样品中成功追溯到了从线性到二次方T2行为的转变,甚至在更低温度下也会发生。此外,过掺杂样品在高温下表现出从线性到对数依赖的转变,这与反铁磁自旋涨落主导电子掺杂铜酸盐的正常态性质相一致。