Powalla Lukas, Kiemle Jonas, König Elio J, Schnyder Andreas P, Knolle Johannes, Kern Klaus, Holleitner Alexander, Kastl Christoph, Burghard Marko
Max-Planck-Institut für Festkörperforschung, Heisenbergstrasse 1, D-70569, Stuttgart, Germany.
Walter Schottky Institut and Physics Department, Technical University of Munich, Am Coulombwall 4a, D-85748, Garching, Germany.
Nat Commun. 2022 Jun 7;13(1):3152. doi: 10.1038/s41467-022-30744-3.
Experimental control of local spin-charge interconversion is of primary interest for spintronics. Van der Waals (vdW) heterostructures combining graphene with a strongly spin-orbit coupled two-dimensional (2D) material enable such functionality by design. Electric spin valve experiments have thus far provided global information on such devices, while leaving the local interplay between symmetry breaking, charge flow across the heterointerface and aspects of topology unexplored. Here, we probe the gate-tunable local spin polarisation in current-driven graphene/WTe heterostructures through magneto-optical Kerr microscopy. Even for a nominal in-plane transport, substantial out-of-plane spin accumulation is induced by a corresponding out-of-plane current flow. We present a theoretical model which fully explains the gate- and bias-dependent onset and spatial distribution of the intense Kerr signal as a result of a non-linear anomalous Hall effect in the heterostructure, which is enabled by its reduced point group symmetry. Our findings unravel the potential of 2D heterostructure engineering for harnessing topological phenomena for spintronics, and constitute an important step toward nanoscale, electrical spin control.
对自旋电子学而言,局部自旋-电荷相互转换的实验控制至关重要。将石墨烯与强自旋轨道耦合二维(2D)材料相结合的范德华(vdW)异质结构通过设计实现了这种功能。迄今为止,电自旋阀实验提供了关于此类器件的全局信息,但尚未探索对称性破缺、异质界面电荷流动与拓扑方面之间的局部相互作用。在此,我们通过磁光克尔显微镜探测电流驱动的石墨烯/WTe异质结构中栅极可调的局部自旋极化。即使对于名义上的面内输运,相应的面外电流也会诱导出大量的面外自旋积累。我们提出了一个理论模型,该模型充分解释了由于异质结构中非线性反常霍尔效应导致的强克尔信号的栅极和偏置依赖性起始及空间分布,这种效应是由其降低的点群对称性实现的。我们的研究结果揭示了二维异质结构工程在利用拓扑现象实现自旋电子学方面的潜力,并朝着纳米级电自旋控制迈出了重要一步。