Wang Qinsheng, Zheng Jingchuan, He Yuan, Cao Jin, Liu Xin, Wang Maoyuan, Ma Junchao, Lai Jiawei, Lu Hong, Jia Shuang, Yan Dayu, Shi Youguo, Duan Junxi, Han Junfeng, Xiao Wende, Chen Jian-Hao, Sun Kai, Yao Yugui, Sun Dong
Key Laboratory of Advanced Optoelectronic Quantum Architecture and Measurement (MOE), School of Physics, Beijing Institute of Technology, Beijing, China.
Micronano Centre, Beijing Key Lab of Nanophotonics & Ultrafine Optoelectronic Systems, Beijing Institute of Technology, Beijing, China.
Nat Commun. 2019 Dec 16;10(1):5736. doi: 10.1038/s41467-019-13713-1.
Photosensing and energy harvesting based on exotic properties of quantum materials and new operation principles have great potential to break the fundamental performance limit of conventional photodetectors and solar cells. Weyl semimetals have demonstrated novel optoelectronic properties that promise potential applications in photodetection and energy harvesting arising from their gapless linear dispersion and Berry field enhanced nonlinear optical effect at the vicinity of Weyl nodes. In this work, we demonstrate robust photocurrent generation at the edge of T-WTe, a type-II Weyl semimetal, due to crystalline-symmetry breaking along certain crystal fracture directions and possibly enhanced by robust fermi-arc type surface states. This edge response is highly generic and arises universally in a wide class of quantum materials with similar crystal symmetries. The robust and generic edge current response provides a charge separation mechanism for photosensing and energy harvesting over broad wavelength range.
基于量子材料的奇异特性和新的工作原理进行的光传感和能量收集,具有突破传统光电探测器和太阳能电池基本性能极限的巨大潜力。外尔半金属已展现出新颖的光电特性,因其无隙线性色散以及在魏尔节点附近的贝里场增强非线性光学效应,有望在光探测和能量收集中得到潜在应用。在这项工作中,我们证明了在II型外尔半金属T-WTe的边缘处能产生稳健的光电流,这是由于沿特定晶体断裂方向的晶体对称性破缺所致,并且可能因稳健的费米弧型表面态而增强。这种边缘响应具有高度普遍性,普遍存在于具有相似晶体对称性的广泛量子材料中。稳健且通用的边缘电流响应为宽波长范围内的光传感和能量收集提供了一种电荷分离机制。