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高熵合金薄膜中的高临界电流密度和高耐受性超导性。

High critical current density and high-tolerance superconductivity in high-entropy alloy thin films.

作者信息

Jung Soon-Gil, Han Yoonseok, Kim Jin Hee, Hidayati Rahmatul, Rhyee Jong-Soo, Lee Jung Min, Kang Won Nam, Choi Woo Seok, Jeon Hye-Ran, Suk Jaekwon, Park Tuson

机构信息

Center for Quantum Materials and Superconductivity (CQMS), Sungkyunkwan University, Suwon, 16419, Republic of Korea.

Department of Physics, Sungkyunkwan University, Suwon, 16419, Republic of Korea.

出版信息

Nat Commun. 2022 Jun 11;13(1):3373. doi: 10.1038/s41467-022-30912-5.

DOI:10.1038/s41467-022-30912-5
PMID:35690593
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC9188561/
Abstract

High-entropy alloy (HEA) superconductors-a new class of functional materials-can be utilized stably under extreme conditions, such as in space environments, owing to their high mechanical hardness and excellent irradiation tolerance. However, the feasibility of practical applications of HEA superconductors has not yet been demonstrated because the critical current density (J) for HEA superconductors has not yet been adequately characterized. Here, we report the fabrication of high-quality superconducting (SC) thin films of Ta-Nb-Hf-Zr-Ti HEAs via a pulsed laser deposition. The thin films exhibit a large J of >1 MA cm at 4.2 K and are therefore favorable for SC devices as well as large-scale applications. In addition, they show extremely robust superconductivity to irradiation-induced disorder controlled by the dose of Kr-ion irradiation. The superconductivity of the HEA films is more than 1000 times more resistant to displacement damage than that of other promising superconductors with technological applications, such as MgB, NbSn, Fe-based superconductors, and high-T cuprate superconductors. These results demonstrate that HEA superconductors have considerable potential for use under extreme conditions, such as in aerospace applications, nuclear fusion reactors, and high-field SC magnets.

摘要

高熵合金(HEA)超导体——一类新型功能材料——由于其高机械硬度和出色的抗辐照能力,能够在极端条件下稳定使用,比如在太空环境中。然而,由于尚未充分表征HEA超导体的临界电流密度(J),其实际应用的可行性尚未得到证实。在此,我们报告了通过脉冲激光沉积制备Ta-Nb-Hf-Zr-Ti HEA高质量超导(SC)薄膜的方法。这些薄膜在4.2 K时表现出大于1 MA/cm²的大临界电流密度(J),因此有利于超导器件以及大规模应用。此外,它们对由氪离子辐照剂量控制的辐照诱导无序表现出极强的超导稳定性。与其他具有技术应用前景的超导体(如MgB₂、Nb₃Sn、铁基超导体和高温铜酸盐超导体)相比,HEA薄膜的超导性对位移损伤的耐受性高出1000倍以上。这些结果表明,HEA超导体在极端条件下(如航空航天应用、核聚变反应堆和高场超导磁体)具有相当大的应用潜力。

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